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Coal and Biomass to Liquid Transportation Fuels: Process Synthesis and Global Optimization Strategies
Alternative TitleInd. Eng. Chem. Res.
Niziolek, Alexander M.1; Onel, Onur1; Elia, Josephine A.1; Baliban, Richard C.1; Xiao, Xin2; Floudas, Christodoulos A.1
2014-11-05
Source PublicationINDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
ISSN0888-5885
Volume53Issue:44Pages:17002-17025
AbstractThe thermochemical conversion of coal and biomass to liquid transportation fuels from a synthesis gas intermediate is investigated using an optimization-based process synthesis framework. Two distinct types of coal (LV bituminous and coal commonly found in the province of Anhui, China) and two types of biomass (hardwood and duckweed) are considered as feedstocks. The superstructure incorporates alternative conversion pathways of synthesis gas which include methanol formation and conversion into FischerTropsch hydrocarbons. Methanol may be converted to gasoline or olefins, and the olefins may be subsequently converted to gasoline and distillate. A rigorous deterministic global optimization branch-and-bound framework is utilized to determine the optimal process topology that produces liquid fuels at the lowest possible cost. Economies of scale are evident as the refinery capacity increases and it is observed that the fuel ratios of the final liquid products have a significant impact on the optimal topology of the plant. The results suggest that liquid fuels production from coal and biomass can be competitive with petroleum-based processes.; The thermochemical conversion of coal and biomass to liquid transportation fuels from a synthesis gas intermediate is investigated using an optimization-based process synthesis framework. Two distinct types of coal (LV bituminous and coal commonly found in the province of Anhui, China) and two types of biomass (hardwood and duckweed) are considered as feedstocks. The superstructure incorporates alternative conversion pathways of synthesis gas which include methanol formation and conversion into FischerTropsch hydrocarbons. Methanol may be converted to gasoline or olefins, and the olefins may be subsequently converted to gasoline and distillate. A rigorous deterministic global optimization branch-and-bound framework is utilized to determine the optimal process topology that produces liquid fuels at the lowest possible cost. Economies of scale are evident as the refinery capacity increases and it is observed that the fuel ratios of the final liquid products have a significant impact on the optimal topology of the plant. The results suggest that liquid fuels production from coal and biomass can be competitive with petroleum-based processes.
KeywordNatural-gas Processes Swine Waste-water Lemna-minor Chemical-processes Tropsch Synthesis Duckweed Biomass Growing Duckweed Dimethyl Ether Hybrid Biomass Co2 Emission
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
DOI10.1021/ie500505h
URL查看原文
Indexed BySCI
Language英语
WOS KeywordNATURAL-GAS PROCESSES ; SWINE WASTE-WATER ; LEMNA-MINOR ; CHEMICAL-PROCESSES ; TROPSCH SYNTHESIS ; DUCKWEED BIOMASS ; GROWING DUCKWEED ; DIMETHYL ETHER ; HYBRID BIOMASS ; CO2 EMISSION
WOS Research AreaEngineering
WOS SubjectEngineering, Chemical
WOS IDWOS:000344516900010
Citation statistics
Cited Times:35[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/11811
Collection研究所(批量导入)
Affiliation1.Princeton Univ, Dept Chem & Biol Engn, Princeton, NJ 08544 USA
2.Chinese Acad Sci, Langfang Engn & Technol Ctr, Natl Engn Lab Hydromet Cleaner Prod Technol, Inst Proc Engn, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Niziolek, Alexander M.,Onel, Onur,Elia, Josephine A.,et al. Coal and Biomass to Liquid Transportation Fuels: Process Synthesis and Global Optimization Strategies[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2014,53(44):17002-17025.
APA Niziolek, Alexander M.,Onel, Onur,Elia, Josephine A.,Baliban, Richard C.,Xiao, Xin,&Floudas, Christodoulos A..(2014).Coal and Biomass to Liquid Transportation Fuels: Process Synthesis and Global Optimization Strategies.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,53(44),17002-17025.
MLA Niziolek, Alexander M.,et al."Coal and Biomass to Liquid Transportation Fuels: Process Synthesis and Global Optimization Strategies".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 53.44(2014):17002-17025.
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