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Thermochemical Conversion of Duckweed Biomass to Gasoline, Diesel, and Jet Fuel: Process Synthesis and Global Optimization
Baliban, Richard C.1; Elia, Josephine A.1; Floudas, Christodoulos A.1; Xiao, Xin2; Zhang, Zhijian3; Li, Jie4; Cao, Hongbin5; Ma, Jiong3; Qiao, Yong6; Hu, Xuteng7
2013-08-21
Source PublicationINDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
Volume52Issue:33Pages:11436-11450
AbstractDuckweed biomass is gasified in a thermochemical-based superstructure to produce gasoline, diesel, and kerosene using a synthesis gas intermediate. The superstructure includes multiple pathways for conversion of the synthesis gas to liquid hydrocarbons via Fischer-Tropsch synthesis or intermediate methanol synthesis. Low-temperature and high-temperature Fischer-Tropsch processes are examined using both iron and cobalt based catalysts. Methanol may be converted to hydrocarbons via the methanol-to-gasoline or methanol-to-olefins processes. The hydrocarbons will be refined into the final liquid products using ZSM-5 catalytic conversion, oligomerization, alkylation, isomerization, hydrotreating, reforming, and hydrocracking. A process synthesis framework is outlined to select the refining pathway that will produce the liquid fuels as the lowest possible cost. A rigorous deterministic branch-and-bound global optimization strategy will be incorporated to theoretically guarantee that the overall cost of the solution chosen by the synthesis framework is within a small fraction of the best possible value. A heat, power, and water integration is incorporated within the process synthesis framework to ensure that the cost of utility production and wastewater treatment are simultaneously included with the synthesis of the core refining processes. The proposed process synthesis framework is demonstrated using four case studies which determine the effect of refinery capacity and liquid fuel composition on the overall system cost, the refinery topological design, the process material/energy balances, and the life cycle greenhouse gas emissions.
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
Indexed BySCI
Language英语
WOS KeywordSWINE WASTE-WATER ; LEMNA-MINOR ; GROWING DUCKWEED ; NATURAL-GAS ; ANIMAL FEED ; ENERGY ; ETHANOL ; HYBRID ; PRETREATMENT ; BIOETHANOL
WOS Research AreaEngineering
WOS SubjectEngineering, Chemical
WOS IDWOS:000323536000021
Citation statistics
Cited Times:58[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/13439
Collection研究所(批量导入)
Affiliation1.Princeton Univ, Dept Chem & Biol Engn, Princeton, NJ 08544 USA
2.Chinese Acad Sci, Inst Proc Engn, Langfang Engn & Technol Ctr, Beijing 100190, Peoples R China
3.Peking Univ, Sch Environm & Energy, Shenzhen Grad Sch, Shenzhen 518055, Peoples R China
4.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
5.Chinese Acad Sci, Inst Proc Engn, Res Ctr Proc Pollut Control, Beijing 100190, Peoples R China
6.PetroChina Co Ltd, Sci Technol & Informat Dept, PetroChina Refining & Chem Co, Beijing 100007, Peoples R China
7.PetroChina Co Ltd, Petrochem Res Inst, Beijing 100195, Peoples R China
Recommended Citation
GB/T 7714
Baliban, Richard C.,Elia, Josephine A.,Floudas, Christodoulos A.,et al. Thermochemical Conversion of Duckweed Biomass to Gasoline, Diesel, and Jet Fuel: Process Synthesis and Global Optimization[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2013,52(33):11436-11450.
APA Baliban, Richard C..,Elia, Josephine A..,Floudas, Christodoulos A..,Xiao, Xin.,Zhang, Zhijian.,...&Hu, Xuteng.(2013).Thermochemical Conversion of Duckweed Biomass to Gasoline, Diesel, and Jet Fuel: Process Synthesis and Global Optimization.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,52(33),11436-11450.
MLA Baliban, Richard C.,et al."Thermochemical Conversion of Duckweed Biomass to Gasoline, Diesel, and Jet Fuel: Process Synthesis and Global Optimization".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 52.33(2013):11436-11450.
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