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Interactions of Supercritical CO2 with Coal
Zhang, Dengfeng1; Gu, Lili1; Li, Songgeng2; Lian, Peichao1; Tao, Jun1
2013
Source PublicationENERGY & FUELS
Volume27Issue:1Pages:387-393
AbstractCarbon dioxide sequestration on coal with enhanced coalbed methane recovery (CO2-ECBM) is acknowledged as a promising way to mitigate CO2 emissions. For successfully understanding and implementing CO2-ECBM process, the potential interactions of CO2 with coal during CO2 sequestration in coal seams were investigated. Research methods consisting of low-temperature nitrogen adsorption desorption and chromatographic analysis were used to address the transformation of coal pore morphology and the capability of supercritical CO2 extraction when coal contacts with high pressure CO2. According to the test results, interaction of coal with high pressure CO2 does not create a significant influence on pore shape and mesoporous volume distribution of any rank of coal. However, this causes the coal surface fractal dimension and specific surface area to be changed, which implies that the coal's pore morphology change due to CO2 sorption is irreversible. The results also indicate that the injection of high-pressure CO2 does not only change the pore morphology of coal but also has the ability to extract the hydrocarbons present in the coal matrix. The extracted hydrocarbons are of biological toxicity and can be mobilized with gas or water to other geologic structures and aquifers. Thus, the potential environmental safety and health issues (ES&H issues) related to CO2 sequestration in deep coal seams require thorough assessment.
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
Indexed BySCI
Language英语
WOS KeywordCARBON-DIOXIDE ; TRANSPORT-PROPERTIES ; METHANE RECOVERY ; PORE STRUCTURE ; GAS-PRESSURE ; ADSORPTION ; SORPTION ; SURFACES ; SEQUESTRATION ; PERMEABILITY
WOS Research AreaEnergy & Fuels ; Engineering
WOS SubjectEnergy & Fuels ; Engineering, Chemical
WOS IDWOS:000317327700045
Citation statistics
Cited Times:43[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/13718
Collection研究所(批量导入)
Affiliation1.Kunming Univ Sci & Technol, Fac Chem Engn, Kunming 650500, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Dengfeng,Gu, Lili,Li, Songgeng,et al. Interactions of Supercritical CO2 with Coal[J]. ENERGY & FUELS,2013,27(1):387-393.
APA Zhang, Dengfeng,Gu, Lili,Li, Songgeng,Lian, Peichao,&Tao, Jun.(2013).Interactions of Supercritical CO2 with Coal.ENERGY & FUELS,27(1),387-393.
MLA Zhang, Dengfeng,et al."Interactions of Supercritical CO2 with Coal".ENERGY & FUELS 27.1(2013):387-393.
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