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Upgrading Shale Oil Distillation to Clean Fuel by Coupled Hydrogenation and Ring Opening Reaction of Aromatics on W-Ni/gamma-Al2O3 Catalysts
Wang, Hongyan1,2; Dai, Fei1,2; Li, Zengxi1; Li, Chunshan2
2015-08-01
Source PublicationENERGY & FUELS
ISSN0887-0624
Volume29Issue:8Pages:4902-4910
AbstractTo obtain clean liquid fuel, a study was conducted on upgrading shale oil by hydroconversion. Various W-Ni catalysts were synthesized and characterized using XRD, BET, TG, H-2-TPR, and NH3-TPD methods. The effects of tungsten content and calcination temperature on the physicochemical properties and activity of catalysts were systematically investigated. W-Ni/Al2O3 with 15 wt % W-loading and 550 degrees C calcination temperature was selected as the optimized catalyst. The product distribution of the primary aromatics in shale oil affected by hydrogenation, ring opening, and cracking reactions was discussed. Finally, key reaction parameters such as pressure, liquid hourly space velocity, and H-2/oil volume ratio were optimized. Characteristics of gasoline and diesel fractions were also measured.
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
DOI10.1021/acs.energyfuels.5b01060
Indexed BySCI
Language英语
WOS KeywordTEMPERATURE COAL-TAR ; IONIC LIQUIDS ; HEAVY OILS ; KINETICS ; HYDRODENITROGENATION ; HYDRODESULFURIZATION ; HYDRODEOXYGENATION ; HYDROTREATMENT ; HYDROCARBONS ; EXTRACTION
WOS Research AreaEnergy & Fuels ; Engineering
WOS SubjectEnergy & Fuels ; Engineering, Chemical
WOS IDWOS:000360026700026
Citation statistics
Cited Times:17[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/19484
Collection研究所(批量导入)
Affiliation1.Univ Chinese Acad Sci, Coll Chem & Chem Engn, Beijing 100049, Peoples R China
2.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, Inst Proc Engn, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Wang, Hongyan,Dai, Fei,Li, Zengxi,et al. Upgrading Shale Oil Distillation to Clean Fuel by Coupled Hydrogenation and Ring Opening Reaction of Aromatics on W-Ni/gamma-Al2O3 Catalysts[J]. ENERGY & FUELS,2015,29(8):4902-4910.
APA Wang, Hongyan,Dai, Fei,Li, Zengxi,&Li, Chunshan.(2015).Upgrading Shale Oil Distillation to Clean Fuel by Coupled Hydrogenation and Ring Opening Reaction of Aromatics on W-Ni/gamma-Al2O3 Catalysts.ENERGY & FUELS,29(8),4902-4910.
MLA Wang, Hongyan,et al."Upgrading Shale Oil Distillation to Clean Fuel by Coupled Hydrogenation and Ring Opening Reaction of Aromatics on W-Ni/gamma-Al2O3 Catalysts".ENERGY & FUELS 29.8(2015):4902-4910.
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