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Self-Assembly Reduced Graphene Oxide Nanosheet Hydrogel Fabrication by Anchorage of Chitosan/Silver and Its Potential Efficient Application toward Dye Degradation for Wastewater Treatments
Jiao, Tifeng1,2,3; Zhao, Heng2; Zhou, Jingxin2; Zhang, Qingrui2; Luo, Xiaona2; Hu, Jie2; Peng, Qiuming1; Yan, Xuehai3
2015-12-01
发表期刊ACS SUSTAINABLE CHEMISTRY & ENGINEERING
ISSN2168-0485
卷号3期号:12页码:3130-3139
摘要In this study, the hydrogel materials of reduced graphene oxide (RGO)/chitosan/silver nanoparticle composites were designed and prepared via a self-assembly process and simultaneous reduction of chitosan molecules with GO. These as-prepared hydrogels were characterized by different techniques. The morphology of the internal network structure of the nanocomposite hydrogels was investigated. The catalytic capacity results demonstrate that the prepared GO-based composite hydrogels can efficiently remove two tested dye molecules from wastewater in good accordance with the pseudo-second-order model. The dye photocatalytic capacity of the obtained hydrogels is mainly attributed to the silver nanoparticle on RGO sheets, whereas the chitosan molecule was incorporated to facilitate the gelation process of the GO sheets. Interestingly, the as-prepared catalytic composite material serves as a good photocatalyst for two presently used dyes even for dye mixtures, suggesting the potentially real applications of the GO composite materials for wastewater treatment as well as the removal of harmful dyes.
关键词Graphene Oxide Composite Hydrogel Chitosan Dye Degradation Wastewater Treatment
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1021/acs.suschemeng.5b00695
收录类别SCI
语种英语
关键词[WOS]RAMAN-SPECTRA ; ASYMMETRIC SUPERCAPACITORS ; PHOTOCATALYTIC PERFORMANCE ; SUPRAMOLECULAR HYDROGELS ; CONTROLLED-RELEASE ; ORGANIC POLLUTANT ; AQUEOUS-SOLUTION ; METHYLENE-BLUE ; GRAPHITE OXIDE ; NANOCOMPOSITE
WOS研究方向Chemistry ; Engineering
WOS类目Chemistry, Multidisciplinary ; Engineering, Chemical
项目资助者NSFC(21473153 ; NSF of Hebei Province(B2013203108) ; Science Foundation for the Excellent Youth Scholars from Universities and Colleges of Hebei Province(YQ2013026) ; Support Program for the Top Young Talents of Hebei Province ; Scientific and Technological Research and Development Program of Qinhuangdao City(201502A006) ; Open Foundation of National Key Laboratory of Biochemical Engineering (Institute of Process Engineering, Chinese Academy of Sciences) ; Key Laboratory of Reservoir Aquatic Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Science(RAE2014CE03B) ; 21207112 ; 51578476)
WOS记录号WOS:000366153700015
引用统计
被引频次:56[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/20148
专题生化工程国家重点实验室
作者单位1.Yanshan Univ, State Key Lab Metastable Mat Sci & Technol, Qinhuangdao 066004, Peoples R China
2.Yanshan Univ, Sch Environm & Chem Engn, Hebei Key Lab Appl Chem, Qinhuangdao 066004, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, Natl Key Lab Biochem Engn, Beijing 100190, Peoples R China
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Jiao, Tifeng,Zhao, Heng,Zhou, Jingxin,et al. Self-Assembly Reduced Graphene Oxide Nanosheet Hydrogel Fabrication by Anchorage of Chitosan/Silver and Its Potential Efficient Application toward Dye Degradation for Wastewater Treatments[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2015,3(12):3130-3139.
APA Jiao, Tifeng.,Zhao, Heng.,Zhou, Jingxin.,Zhang, Qingrui.,Luo, Xiaona.,...&Yan, Xuehai.(2015).Self-Assembly Reduced Graphene Oxide Nanosheet Hydrogel Fabrication by Anchorage of Chitosan/Silver and Its Potential Efficient Application toward Dye Degradation for Wastewater Treatments.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,3(12),3130-3139.
MLA Jiao, Tifeng,et al."Self-Assembly Reduced Graphene Oxide Nanosheet Hydrogel Fabrication by Anchorage of Chitosan/Silver and Its Potential Efficient Application toward Dye Degradation for Wastewater Treatments".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 3.12(2015):3130-3139.
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