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Synthesis and Characterization of Tetramethylethylenediamine-Based Hypergolic Ionic Liquids
Fei, Teng; Cai, Huiwu; Zhang, Yanqiang2; Liu, Long; Zhang, Suojiang
2016-04-02
发表期刊JOURNAL OF ENERGETIC MATERIALS
ISSN0737-0652
卷号34期号:2页码:138-151
摘要Four energetic salts (including two ionic liquids) based on 2-(dimethylamino)-N,N,N-trimethylethanaminium and N,N-dialkyl-N,N,N,N-tetramethylethane-1,2-diaminium was prepared and characterized by H-1- and C-13-NMR, infrared and Raman spectroscopies, and elemental analysis. Their physicochemical properties such as melting and decomposition temperatures, density, viscosity, heat of formation, detonation performance, and specific impulse were measured or calculated. With thermal stability up to 200 degrees C, the resulting ionic liquids show densities from 1.02 to 1.19 g cm(-3) and heats of formation from 85.1 to 154.4 kJ mol(-1). Moreover, 2-(dimethylamino)-N,N,N-trimethylethanaminium dicyanamide is hypergolic with the oxidizer (100% HNO3) and exhibits potential as a green fuel for bipropellants.
关键词Dicyanamide Heat Of Formation Hypergolic Specific Impulse Tetramethylethylenediamine
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1080/07370652.2015.1017669
收录类别SCI
语种英语
关键词[WOS]ENERGETIC SALTS ; FLUIDS ; CATION ; FUELS
WOS研究方向Chemistry ; Engineering ; Materials Science
WOS类目Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical ; Materials Science, Multidisciplinary
项目资助者National Natural Science Foundation of China(21376252 ; National Defense Science and Technology Innovation Fund of Chinese Academy of Sciences(CXJJ-14-M37 ; 21406242) ; CXJJ-14-M41)
WOS记录号WOS:000367067200004
引用统计
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/20190
专题多相复杂系统国家重点实验室
作者单位1.Xian Univ Sci & Technol, Sch Chem & Chem Engn, Xian, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, Beijing Key Lab Ion Liquids Clean Proc, Beijing 100190, Peoples R China
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Fei, Teng,Cai, Huiwu,Zhang, Yanqiang,et al. Synthesis and Characterization of Tetramethylethylenediamine-Based Hypergolic Ionic Liquids[J]. JOURNAL OF ENERGETIC MATERIALS,2016,34(2):138-151.
APA Fei, Teng,Cai, Huiwu,Zhang, Yanqiang,Liu, Long,&Zhang, Suojiang.(2016).Synthesis and Characterization of Tetramethylethylenediamine-Based Hypergolic Ionic Liquids.JOURNAL OF ENERGETIC MATERIALS,34(2),138-151.
MLA Fei, Teng,et al."Synthesis and Characterization of Tetramethylethylenediamine-Based Hypergolic Ionic Liquids".JOURNAL OF ENERGETIC MATERIALS 34.2(2016):138-151.
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