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Electrodeposition of crystalline silicon directly from silicon tetrachloride in ionic liquid at low temperature
Zhang, Junling; Chen, Shimou; Zhang, Haitao; Zhang, Suojiang; Yao, Xue; Shi, Zhaohui
2016
发表期刊RSC ADVANCES
ISSN2046-2069
卷号6期号:15页码:12061-12067
摘要Crystalline silicon (Si) is widely used in modern electronics. Si is commonly produced through a series of energy-intensive reactions (> 700 degrees C). It is thus urgent and significant to explore more economically and environmentally-benign synthetic strategies for crystalline Si at low temperature. In this contribution, we report an efficient method to prepare crystalline Si from silicon tetrachloride at the low temperature of 100 degrees C with an ionic liquid (IL) as electrolyte. Physicochemical characterization revealed that as-deposited crystalline Si with a diamond cubic crystal structure exhibited a dominant (111)-orientation. Moreover, in-depth insights into the growth mechanism of crystalline Si was shed light upon herein. Furthermore, the smart electrodepositing platform of crystalline Si from ILs would open up a new avenue for low-temperature metallurgy of Si.
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
DOI10.1039/c5ra23085c
收录类别SCI
语种英语
关键词[WOS]ELECTROCHEMICAL REDUCTION ; ROOM-TEMPERATURE ; ALUMINUM ELECTRODEPOSITION ; BATTERIES ; CHLORIDE
WOS研究方向Chemistry
WOS类目Chemistry, Multidisciplinary
项目资助者National Basic Research Program of China(2015CB251401) ; National Nature Science Foundations of China(51274181 ; Beijing Municipal Natural Science Foundation(2132054) ; 21276257)
WOS记录号WOS:000369545800018
引用统计
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/20613
专题多相复杂系统国家重点实验室
作者单位Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Key Lab Green Proc & Engn,Inst Proc Engn, Beijing 100190, Peoples R China
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Zhang, Junling,Chen, Shimou,Zhang, Haitao,et al. Electrodeposition of crystalline silicon directly from silicon tetrachloride in ionic liquid at low temperature[J]. RSC ADVANCES,2016,6(15):12061-12067.
APA Zhang, Junling,Chen, Shimou,Zhang, Haitao,Zhang, Suojiang,Yao, Xue,&Shi, Zhaohui.(2016).Electrodeposition of crystalline silicon directly from silicon tetrachloride in ionic liquid at low temperature.RSC ADVANCES,6(15),12061-12067.
MLA Zhang, Junling,et al."Electrodeposition of crystalline silicon directly from silicon tetrachloride in ionic liquid at low temperature".RSC ADVANCES 6.15(2016):12061-12067.
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