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Biomass-Water Interaction and Its Correlations with Enzymatic Hydrolysis of Steam-Exploded Corn Stover
Liu, Zhi-Hua1,2; Chen, Hong-Zhang1
2016-03-01
Source PublicationACS SUSTAINABLE CHEMISTRY & ENGINEERING
ISSN2168-0485
Volume4Issue:3Pages:1274-1285
Abstract

Author: Biomass water interaction is a main factor affecting the enzymatic hydrolysis process. The interactions between corn stover and water and their correlations with enzymatic hydrolysis performance were investigated. The peak height of the main water pool was lower, peak width at half-height was bigger, and T2 relaxation time was shorter in steam-exploded corn stover (SECS) than in untreated corn stover (UCS). The relations between the total peak area of water pools and the moisture content can be well expressed by exponential models. Steam explosion enhanced corn stover water interactions due to an increase in specific surface area, pore volume, average pore diameter, porosity, and oxygen to carbon ratio. Small particle size strengthened UCS water interactions while slightly weakening SECS water interactions. In enzymatic hydrolysis, constrained water was released before 36 h, which was consistent with the increase in glucan conversion. The release of constrained water and increase in glucan conversion facilitated each other. Steam explosion enhanced the interactions between SECS and water (mainly bound water), which increased the accessibility of carbohydrates to enzymes. Therefore, the release of constrained water before 36 h and the increase in SECS water interactions on the surface of SECS facilitated the enzymatic hydrolysis efficiency.

KeywordBiomass-water Interactions Steam Explosion Enzymatic Hydrolysis Water Pool Time Domain Nuclear Magnetic Resonance (Td-nmr) Particle Size
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1021/acssuschemeng.5b01303
Indexed BySCI
Language英语
WOS KeywordNuclear-magnetic-resonance ; Lignocellulosic Biomass ; Solids Loadings ; Particle-size ; Wheat-straw ; Pretreatment ; Cellulose ; Saccharification ; Digestibility ; Accessibility
WOS Research AreaChemistry ; Engineering
WOS SubjectChemistry, Multidisciplinary ; Engineering, Chemical
Funding OrganizationNational High Technology Research and Development Program of China (863 Program)(SS2012AA022502) ; National Key Laboratory of Biochemical Engineering(2013KF-01)
WOS IDWOS:000371755400078
Citation statistics
Cited Times:11[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/20622
Collection研究所(批量导入)
Corresponding AuthorChen, Hong-Zhang
Affiliation1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Liu, Zhi-Hua,Chen, Hong-Zhang. Biomass-Water Interaction and Its Correlations with Enzymatic Hydrolysis of Steam-Exploded Corn Stover[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2016,4(3):1274-1285.
APA Liu, Zhi-Hua,&Chen, Hong-Zhang.(2016).Biomass-Water Interaction and Its Correlations with Enzymatic Hydrolysis of Steam-Exploded Corn Stover.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,4(3),1274-1285.
MLA Liu, Zhi-Hua,et al."Biomass-Water Interaction and Its Correlations with Enzymatic Hydrolysis of Steam-Exploded Corn Stover".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 4.3(2016):1274-1285.
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