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Preparation of steam activated carbon from black liquor by flue gas precipitation and its performance in hydrogen sulfide removal: Experimental and simulation works
Zhang, Jing Ping1; Sun, Yong2; Woo, Meng Wai3; Zhang, Lian3; Xu, Kang Zhen4
2016-02-01
Source PublicationJOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS
ISSN1876-1070
Volume59Issue:FEBPages:395-404
Abstract

Activated carbon was prepared from black liquor by steam activation. The BET specific surface area, pore volume and average pore diameter of resultant carbon activated at 900 degrees C can reach 1010 m(2)/g, 0.65 m(3)/g and 3 nm respectively. The relative humidity contributes to the adsorption of H2S on carbon, while the increased adsorption temperature and inlet concentration show an unfavorable condition for adsorption. Kinetic model yield a satisfactory result in parameters estimation and prediction for breakthrough time with different inlet H2S concentrations. The surface diffusion is significant to the effective diffusivity during mass transfer under experimental condition. The dynamic experimental results indicate a good performance in H2S removal. (C) 2015 Taiwan Institute of Chemical Engineers. Published by Elsevier B.V. All rights reserved.

KeywordLignin Activated Carbon Hydrogen Sulfide Kinetic Modeling Breakthrough Curves
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
DOI10.1016/j.jtice.2015.09.005
URL查看原文
Indexed BySCI
Language英语
WOS KeywordSurface-area ; H3po4 Activation ; Water Pollutants ; Mass-transfer ; Lignin ; Adsorption ; Sulfur ; Model ; Sorbent ; Waste
WOS Research AreaEngineering
WOS SubjectEngineering, Chemical
Funding OrganizationNational High Technology Research and Development Program 863(2011AA060703) ; Innovation funds of institute of processes engineering of Chinese Academy of Sciences(062702)
WOS IDWOS:000370883900047
Citation statistics
Cited Times:25[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/20656
Collection研究所(批量导入)
Corresponding AuthorSun, Yong
Affiliation1.Chinese Acad Sci, Inst Proc Engn, Natl Engn Lab Cleaner Prod Technol, Beijing 100190, Peoples R China
2.CSIRO, Earth Sci & Resources Engn, 26 Dick Perry Ave, Kensington, WA 6151, Australia
3.Monash Univ, Dept Chem Engn, Melbourne, Vic 3800, Australia
4.Northwest Univ, Sch Chem Engn, Xian 710069, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Jing Ping,Sun, Yong,Woo, Meng Wai,et al. Preparation of steam activated carbon from black liquor by flue gas precipitation and its performance in hydrogen sulfide removal: Experimental and simulation works[J]. JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS,2016,59(FEB):395-404.
APA Zhang, Jing Ping,Sun, Yong,Woo, Meng Wai,Zhang, Lian,&Xu, Kang Zhen.(2016).Preparation of steam activated carbon from black liquor by flue gas precipitation and its performance in hydrogen sulfide removal: Experimental and simulation works.JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS,59(FEB),395-404.
MLA Zhang, Jing Ping,et al."Preparation of steam activated carbon from black liquor by flue gas precipitation and its performance in hydrogen sulfide removal: Experimental and simulation works".JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS 59.FEB(2016):395-404.
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