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Experimental and theoretical studies on hydrogen bond-promoted fixation of carbon dioxide and epoxides in cyclic carbonates
Wang, JQ; Sun, J; Cheng, WG; Dong, K; Zhang, XP; Zhang, SJ; Wang, Jin-Quan; Sun, Jian; Cheng, Wei-Guo; Dong, Kun; Zhang, Xiang-Ping; Zhang, Suo-Jiang
2012
发表期刊PHYSICAL CHEMISTRY CHEMICAL PHYSICS
ISSN1463-9076
卷号14期号:31页码:11021
摘要

The hydrogen bond donor-promoted fixation of CO2 and epoxides into cyclic carbonates was investigated through experimental and density functional theory studies. A highly effective homogeneous system of 1,2-benzenediol-tetrabutyl ammonium bromide (TBAB) and heterogeneous poly-ionic liquids were developed for the fixation of CO2 into cyclic carbonates via hydrogen bond activation, based on the understanding of the reaction mechanism and catalyst design. The work hence provides a molecular level understanding of the reaction process and forms the basis for the rational design of catalytic systems for the fixation of CO2 into useful organic compounds.

关键词Ionic Liquids Supercritical Conditions Catalytic-activity Propylene-oxide Ethylene-oxide Co2 Cycloaddition Transformation Capture Silica
文章类型Article
学科领域Chemistry, Physical ; Physics, Atomic, Molecular & Chemical ; Chemistry ; Physics
DOI10.1039/c2cp41698k
URL查看原文
收录类别SCI
语种英语
资助项目National Basic Research Program of China [2009CB219904] ; National Natural Sciences Foundation of China [21003129, 21036007, 20936005]
WOS记录号WOS:000306572600024
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被引频次:72[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/20716
专题研究所(批量导入)
通讯作者Zhang, Suo-Jiang
推荐引用方式
GB/T 7714
Wang, JQ,Sun, J,Cheng, WG,et al. Experimental and theoretical studies on hydrogen bond-promoted fixation of carbon dioxide and epoxides in cyclic carbonates[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2012,14(31):11021.
APA Wang, JQ.,Sun, J.,Cheng, WG.,Dong, K.,Zhang, XP.,...&Zhang, Suo-Jiang.(2012).Experimental and theoretical studies on hydrogen bond-promoted fixation of carbon dioxide and epoxides in cyclic carbonates.PHYSICAL CHEMISTRY CHEMICAL PHYSICS,14(31),11021.
MLA Wang, JQ,et al."Experimental and theoretical studies on hydrogen bond-promoted fixation of carbon dioxide and epoxides in cyclic carbonates".PHYSICAL CHEMISTRY CHEMICAL PHYSICS 14.31(2012):11021.
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