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Pyrolysis of low rank coal by nickel based zeolite catalysts in the two-staged bed reactor
Amin, Muhammad Nadeem; Li, Yi; Razzaq, Rauf; Lu, Xingmei; Li, Chunshan; Zhang, Suojiang
2016-03-01
Source PublicationJOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS
ISSN0165-2370
Volume118Issue:MARPages:54-62
AbstractPyrolysis is an important process in the coal conversion and has a significant effect on the distribution of volatile products. In this work, ZSM-5 zeolite with different Ni loading was studied to upgrade volatile matter using low rank coal (Shengli, Inner Mongolia) in the two-staged bed reactor. All prepared catalysts were characterized using X-ray diffraction (XRD), Brunauer-Emmett-Teller (BET) analysis and ammonia temperature-programmed desorption (NH3-TPD). The role of Ni metal loading toward the pyrolysis gas yield and upgraded pyrolysis oil was investigated. The yield of non-condensable gases decreases as Ni loading increased in the catalysts, especially the yield of CO2 decreased significantly. Moreover, the catalysts reduced the pitch contents in the pyrolysis oil and promoted the fraction of light pyrolysis oils (BP < 360 degrees C). (C) 2016 Elsevier B.V. All rights reserved.
KeywordCoal Pyrolysis Low Rank Coal Catalyst Nickel
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1016/j.jaap.2015.11.019
Indexed BySCI
Language英语
WOS KeywordBITUMINOUS COAL ; FLUIDIZED-BED ; TAR ; GASIFICATION ; BIOMASS ; LIGNITE ; NI
WOS Research AreaChemistry ; Spectroscopy
WOS SubjectChemistry, Analytical ; Spectroscopy
Funding OrganizationBeijing Natural Science Foundation(3142020) ; International S & T Cooperation Program of China(2014DFA61670) ; National Major Instrumentation Development(2011YQ12003907) ; Chinese Academy of Sciences(XDA07010300)
WOS IDWOS:000373541400006
Citation statistics
Cited Times:14[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/20994
Collection多相复杂系统国家重点实验室
AffiliationChinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, Inst Proc Engn, Key Lab Green Proc & Engn,State Key Lab Multiphas, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Amin, Muhammad Nadeem,Li, Yi,Razzaq, Rauf,et al. Pyrolysis of low rank coal by nickel based zeolite catalysts in the two-staged bed reactor[J]. JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS,2016,118(MAR):54-62.
APA Amin, Muhammad Nadeem,Li, Yi,Razzaq, Rauf,Lu, Xingmei,Li, Chunshan,&Zhang, Suojiang.(2016).Pyrolysis of low rank coal by nickel based zeolite catalysts in the two-staged bed reactor.JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS,118(MAR),54-62.
MLA Amin, Muhammad Nadeem,et al."Pyrolysis of low rank coal by nickel based zeolite catalysts in the two-staged bed reactor".JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS 118.MAR(2016):54-62.
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