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Pyrolysis of low rank coal by nickel based zeolite catalysts in the two-staged bed reactor
Amin, Muhammad Nadeem; Li, Yi; Razzaq, Rauf; Lu, Xingmei; Li, Chunshan; Zhang, Suojiang
2016-03-01
发表期刊JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS
ISSN0165-2370
卷号118期号:MAR页码:54-62
摘要Pyrolysis is an important process in the coal conversion and has a significant effect on the distribution of volatile products. In this work, ZSM-5 zeolite with different Ni loading was studied to upgrade volatile matter using low rank coal (Shengli, Inner Mongolia) in the two-staged bed reactor. All prepared catalysts were characterized using X-ray diffraction (XRD), Brunauer-Emmett-Teller (BET) analysis and ammonia temperature-programmed desorption (NH3-TPD). The role of Ni metal loading toward the pyrolysis gas yield and upgraded pyrolysis oil was investigated. The yield of non-condensable gases decreases as Ni loading increased in the catalysts, especially the yield of CO2 decreased significantly. Moreover, the catalysts reduced the pitch contents in the pyrolysis oil and promoted the fraction of light pyrolysis oils (BP < 360 degrees C). (C) 2016 Elsevier B.V. All rights reserved.
关键词Coal Pyrolysis Low Rank Coal Catalyst Nickel
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.jaap.2015.11.019
收录类别SCI
语种英语
关键词[WOS]BITUMINOUS COAL ; FLUIDIZED-BED ; TAR ; GASIFICATION ; BIOMASS ; LIGNITE ; NI
WOS研究方向Chemistry ; Spectroscopy
WOS类目Chemistry, Analytical ; Spectroscopy
项目资助者Beijing Natural Science Foundation(3142020) ; International S & T Cooperation Program of China(2014DFA61670) ; National Major Instrumentation Development(2011YQ12003907) ; Chinese Academy of Sciences(XDA07010300)
WOS记录号WOS:000373541400006
引用统计
被引频次:10[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/20994
专题多相复杂系统国家重点实验室
作者单位Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, Inst Proc Engn, Key Lab Green Proc & Engn,State Key Lab Multiphas, Beijing 100190, Peoples R China
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Amin, Muhammad Nadeem,Li, Yi,Razzaq, Rauf,et al. Pyrolysis of low rank coal by nickel based zeolite catalysts in the two-staged bed reactor[J]. JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS,2016,118(MAR):54-62.
APA Amin, Muhammad Nadeem,Li, Yi,Razzaq, Rauf,Lu, Xingmei,Li, Chunshan,&Zhang, Suojiang.(2016).Pyrolysis of low rank coal by nickel based zeolite catalysts in the two-staged bed reactor.JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS,118(MAR),54-62.
MLA Amin, Muhammad Nadeem,et al."Pyrolysis of low rank coal by nickel based zeolite catalysts in the two-staged bed reactor".JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS 118.MAR(2016):54-62.
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