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Interactive Matching between the Temperature Profile and Secondary Reactions of Oil Shale Pyrolysis
Zhang, Yu1,2; Han, Zhennan1,2; Wu, Hao3; Lai, Dengguo1,2; Glarborg, Peter3; Xu, Guangwen1
2016-04-01
发表期刊ENERGY & FUELS
ISSN0887-0624
卷号30期号:4页码:2865-2873
摘要This article investigates the effect of the reactor temperature profile on the distribution and characteristics of the products from fixed-bed pyrolysis of oil shale. Experiments were performed in a one-stage fixed-bed reactor and in a two-stage fixed-bed reactor. In the one-stage reactor, the shale oil yield reached 7.40 wt % with a reactor temperature profile from 900 to 550 degrees C and decreased to 2.23 wt % with the reverse temperature profile. The effect of the temperature profile was investigated further in the two-stage fixed-bed reactor combining a pyrolysis stage operating at 550 degrees C and a shale char bed operating at different temperatures. At low temperatures (<450 degrees C) in the shale char bed, the primary oil from the pyrolysis reactor condensed. The condensed oil was released once the bed was reheated to 550 degrees C, thus causing a slight oil loss but a higher yield of light oil (boiling point <350 degrees C) due to oil cracking over the shale char. At high temperatures in the shale char bed (>550 degrees C), severe cracking occurred, converting both heavy and light oil to carbon and gas. The desirably matched reactor temperature profile for high oil yield is discussed via analysis of the tendency of secondary reactions subject to the temperature of particles contacting primary volatiles.
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1021/acs.energyfuels.6b00227
收录类别SCI
语种英语
关键词[WOS]SOLID HEAT CARRIER ; COMPREHENSIVE UTILIZATION ; COAL PYROLYSIS ; FIXED-BED ; CRACKING ; INTERNALS ; KINETICS ; PERFORMANCE ; ZEOLITE ; CARBON
WOS研究方向Energy & Fuels ; Engineering
WOS类目Energy & Fuels ; Engineering, Chemical
项目资助者National Basic Research Program of China(2014CB744303) ; National Natural Science Foundation of China(91534125)
WOS记录号WOS:000374804400035
引用统计
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/21044
专题多相复杂系统国家重点实验室
作者单位1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Tech Univ Denmark, Dept Chem & Biochem Engn, Lyngby Campus, DK-2800 Lyngby, Denmark
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Zhang, Yu,Han, Zhennan,Wu, Hao,et al. Interactive Matching between the Temperature Profile and Secondary Reactions of Oil Shale Pyrolysis[J]. ENERGY & FUELS,2016,30(4):2865-2873.
APA Zhang, Yu,Han, Zhennan,Wu, Hao,Lai, Dengguo,Glarborg, Peter,&Xu, Guangwen.(2016).Interactive Matching between the Temperature Profile and Secondary Reactions of Oil Shale Pyrolysis.ENERGY & FUELS,30(4),2865-2873.
MLA Zhang, Yu,et al."Interactive Matching between the Temperature Profile and Secondary Reactions of Oil Shale Pyrolysis".ENERGY & FUELS 30.4(2016):2865-2873.
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