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Hydrodeoxygenation of phenol over Pd catalysts by in-situ generated hydrogen from aqueous reforming of formic acid
Zeng, Ying1,2; Wang, Ze1; Lin, Weigang1; Song, Wenli1; Christensen, Jakob M.3; Jensen, Anker D.3
2016-07-05
Source PublicationCATALYSIS COMMUNICATIONS
ISSN1566-7367
Volume82Issue:JULYPages:46-49
AbstractHydrodeoxygenation of phenol, as model compound of bio-oil, was investigated over Pd catalysts, using formic acid as a hydrogen donor. The order of activity for deoxygenation of phenol with Pd catalysts was found to be: Pd/SiO2 > Pd/MCM-41 > Pd/CA > Pd/Al2O3 > Pd/HY approximate to Pd/ZrO2 approximate to Pd/CW > Pd/HSAPO-34 > Pd/HZSM-5. The good performance of Pd/SiO2 is owing to its proper pore structure and large specific surface area. The high level of Bronsted acid sites in SiO2 also favors the deoxygenation of phenol. (C) 2016 Elsevier B.V. All rights reserved.
KeywordPhenol Formic Acid In-situ Hydrodeoxygenation Hydrogen Donor
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
DOI10.1016/j.catcom.2016.04.018
Indexed BySCI
Language英语
WOS KeywordBIO-OIL ; MODEL COMPOUNDS ; FUELS
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
Funding OrganizationNational Natural Science Foundation of China(51476180) ; International S&T Cooperation Program of China(2013DFG62640)
WOS IDWOS:000377735500011
Citation statistics
Cited Times:10[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/21156
Collection多相复杂系统国家重点实验室
Affiliation1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Sino Danish Ctr Educ & Res, Beijing 100190, Peoples R China
3.Tech Univ Denmark, Dept Chem & Biochem Engn, Bldg 229, DK-2800 Lyngby, Denmark
Recommended Citation
GB/T 7714
Zeng, Ying,Wang, Ze,Lin, Weigang,et al. Hydrodeoxygenation of phenol over Pd catalysts by in-situ generated hydrogen from aqueous reforming of formic acid[J]. CATALYSIS COMMUNICATIONS,2016,82(JULY):46-49.
APA Zeng, Ying,Wang, Ze,Lin, Weigang,Song, Wenli,Christensen, Jakob M.,&Jensen, Anker D..(2016).Hydrodeoxygenation of phenol over Pd catalysts by in-situ generated hydrogen from aqueous reforming of formic acid.CATALYSIS COMMUNICATIONS,82(JULY),46-49.
MLA Zeng, Ying,et al."Hydrodeoxygenation of phenol over Pd catalysts by in-situ generated hydrogen from aqueous reforming of formic acid".CATALYSIS COMMUNICATIONS 82.JULY(2016):46-49.
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