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Hydrodeoxygenation of phenol over Pd catalysts by in-situ generated hydrogen from aqueous reforming of formic acid
Zeng, Ying1,2; Wang, Ze1; Lin, Weigang1; Song, Wenli1; Christensen, Jakob M.3; Jensen, Anker D.3
2016-07-05
发表期刊CATALYSIS COMMUNICATIONS
ISSN1566-7367
卷号82期号:JULY页码:46-49
摘要Hydrodeoxygenation of phenol, as model compound of bio-oil, was investigated over Pd catalysts, using formic acid as a hydrogen donor. The order of activity for deoxygenation of phenol with Pd catalysts was found to be: Pd/SiO2 > Pd/MCM-41 > Pd/CA > Pd/Al2O3 > Pd/HY approximate to Pd/ZrO2 approximate to Pd/CW > Pd/HSAPO-34 > Pd/HZSM-5. The good performance of Pd/SiO2 is owing to its proper pore structure and large specific surface area. The high level of Bronsted acid sites in SiO2 also favors the deoxygenation of phenol. (C) 2016 Elsevier B.V. All rights reserved.
关键词Phenol Formic Acid In-situ Hydrodeoxygenation Hydrogen Donor
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
DOI10.1016/j.catcom.2016.04.018
收录类别SCI
语种英语
关键词[WOS]BIO-OIL ; MODEL COMPOUNDS ; FUELS
WOS研究方向Chemistry
WOS类目Chemistry, Physical
项目资助者National Natural Science Foundation of China(51476180) ; International S&T Cooperation Program of China(2013DFG62640)
WOS记录号WOS:000377735500011
引用统计
被引频次:7[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/21156
专题多相复杂系统国家重点实验室
作者单位1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Sino Danish Ctr Educ & Res, Beijing 100190, Peoples R China
3.Tech Univ Denmark, Dept Chem & Biochem Engn, Bldg 229, DK-2800 Lyngby, Denmark
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GB/T 7714
Zeng, Ying,Wang, Ze,Lin, Weigang,et al. Hydrodeoxygenation of phenol over Pd catalysts by in-situ generated hydrogen from aqueous reforming of formic acid[J]. CATALYSIS COMMUNICATIONS,2016,82(JULY):46-49.
APA Zeng, Ying,Wang, Ze,Lin, Weigang,Song, Wenli,Christensen, Jakob M.,&Jensen, Anker D..(2016).Hydrodeoxygenation of phenol over Pd catalysts by in-situ generated hydrogen from aqueous reforming of formic acid.CATALYSIS COMMUNICATIONS,82(JULY),46-49.
MLA Zeng, Ying,et al."Hydrodeoxygenation of phenol over Pd catalysts by in-situ generated hydrogen from aqueous reforming of formic acid".CATALYSIS COMMUNICATIONS 82.JULY(2016):46-49.
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