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Coal pyrolysis and its mechanism in indirectly heated fixed-bed with metallic heating plate enhancement
Hu, Erfeng1,2,3; Zhu, Chuanqiang4; Rogers, Kyle3; Han, Xue3; Wang, Jie1; Zhao, Jing1; Fu, Xiaoheng1
2016-12-01
发表期刊FUEL
ISSN0016-2361
卷号185期号:DEC页码:656-662
摘要

A metallic plate has been devised to enhance the heat transfer; this in turn increases the yield and quality of coal tar (Zhang et al., 2013). This work is devoted to investigating the pyrolysis of Yilan subbituminous coal and developing a working mechanism for an indirectly heated fixed bed reactor with different number of metallic plates. Increasing the number of metallic heating plates enhanced the heat transfer from the high-temperature reactor wall to the low-temperature central coal layer and thereby shortened the reaction time. Meanwhile, the yields of tar and light fraction were increased then decreased. The results of the pressure drop experiment demonstrated that the metallic plates weakened dense stacks of coal particles and raised the particle interstices, and therefore lowered the gas diffusion resistance. It verified that many gaseous pyrolysis products escaped from the central low-temperature coal layer, indicating the suppressed secondary reactions to the primary products. When the number of plates was 8, the correspondingly added high-temperature surface was 113%; it achieved the optimal matching between the secondary reactions of pyrolysis products and the fields of the temperature as well as the gas flow inside the reactor, and it also had the highest tar yield (6.60 wt.% dry basis) and the maximum content of light tar (below the boiling points of 360 degrees C) of 76.4 wt.% and C4-C9 components of 43.52 wt.%. The BET results showed that the char had the biggest surface area and volume for this case with 8 plates. Consequently, adding suitable metallic plates into the indirectly heated fixed bed reactor obviously enhances the heat transfer and also achieves higher yield and quality of tar. (C) 2016 Published by Elsevier Ltd.

关键词Coal Pyrolysis Metallic Heating Plates Secondary Reaction Reaction Mechanism
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1016/j.fuel.2016.07.115
收录类别SCI
语种英语
关键词[WOS]WIRE-MESH REACTOR ; VACUUM PYROLYSIS ; PARTICLE-SIZE ; OIL-SHALE ; TEMPERATURE ; TARS ; CHAR ; GASIFICATION ; CONVERSION ; PRESSURE
WOS研究方向Energy & Fuels ; Engineering
WOS类目Energy & Fuels ; Engineering, Chemical
项目资助者"Strategic Priority Research Program" of CAS(XDA07050400) ; State Scholarship Fund of China(201506430030)
WOS记录号WOS:000382248700068
引用统计
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/21312
专题多相复杂系统国家重点实验室
作者单位1.China Univ Min & Technol Beijing, Sch Chem & Environm Engn, Beijing 100083, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
3.Univ New Brunswick, Dept Chem Engn, Fredericton, NB E3B 5A3, Canada
4.China Everbright Int Ltd, Shenzhen 518000, Peoples R China
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Hu, Erfeng,Zhu, Chuanqiang,Rogers, Kyle,et al. Coal pyrolysis and its mechanism in indirectly heated fixed-bed with metallic heating plate enhancement[J]. FUEL,2016,185(DEC):656-662.
APA Hu, Erfeng.,Zhu, Chuanqiang.,Rogers, Kyle.,Han, Xue.,Wang, Jie.,...&Fu, Xiaoheng.(2016).Coal pyrolysis and its mechanism in indirectly heated fixed-bed with metallic heating plate enhancement.FUEL,185(DEC),656-662.
MLA Hu, Erfeng,et al."Coal pyrolysis and its mechanism in indirectly heated fixed-bed with metallic heating plate enhancement".FUEL 185.DEC(2016):656-662.
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