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Core-shell Au-Pd nanoparticles as cathode catalysts for microbial fuel cell applications
Yang, Gaixiu1,2; Chen, Dong3; Lv, Pengmei1,2; Kong, Xiaoying1,2; Sun, Yongming1,2; Wang, Zhongming1,2; Yuan, Zhenhong1,2; Liu, Hui3; Yang, Jun3
2016-10-13
发表期刊SCIENTIFIC REPORTS
ISSN2045-2322
卷号6期号:OCT页码:35252
摘要

Bimetallic nanoparticles with core-shell structures usually display enhanced catalytic properties due to the lattice strain created between the core and shell regions. In this study, we demonstrate the application of bimetallic Au-Pd nanoparticles with an Au core and a thin Pd shell as cathode catalysts in microbial fuel cells, which represent a promising technology for wastewater treatment, while directly generating electrical energy. In specific, in comparison with the hollow structured Pt nanoparticles, a benchmark for the electrocatalysis, the bimetallic core-shell Au-Pd nanoparticles are found to have superior activity and stability for oxygen reduction reaction in a neutral condition due to the strong electronic interaction and lattice strain effect between the Au core and the Pd shell domains. The maximum power density generated in a membraneless single-chamber microbial fuel cell running on wastewater with core-shell Au-Pd as cathode catalysts is ca. 16.0 W m(-3) and remains stable over 150 days, clearly illustrating the potential of core-shell nanostructures in the applications of microbial fuel cells.

文章类型Article
WOS标题词Science & Technology
DOI10.1038/srep35252
收录类别SCI
语种英语
关键词[WOS]OXYGEN REDUCTION REACTION ; ACTIVATED CARBON ; AIR-CATHODE ; PERFORMANCE ; ELECTROCATALYSIS ; TECHNOLOGY ; MEMBRANE ; SYSTEM ; ENERGY ; WASTE
WOS研究方向Science & Technology - Other Topics
WOS类目Multidisciplinary Sciences
项目资助者Science and Technology Service Network Initiative(KFJ-Ew-STS-138) ; Science and Technology Planing Project of Guangdong Province(2015B020241002) ; National Natural Science Foundation of China(21376247 ; 21506225 ; 21573240)
WOS记录号WOS:000385344400001
引用统计
被引频次:8[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/21565
专题多相复杂系统国家重点实验室
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
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GB/T 7714
Yang, Gaixiu,Chen, Dong,Lv, Pengmei,et al. Core-shell Au-Pd nanoparticles as cathode catalysts for microbial fuel cell applications[J]. SCIENTIFIC REPORTS,2016,6(OCT):35252.
APA Yang, Gaixiu.,Chen, Dong.,Lv, Pengmei.,Kong, Xiaoying.,Sun, Yongming.,...&Yang, Jun.(2016).Core-shell Au-Pd nanoparticles as cathode catalysts for microbial fuel cell applications.SCIENTIFIC REPORTS,6(OCT),35252.
MLA Yang, Gaixiu,et al."Core-shell Au-Pd nanoparticles as cathode catalysts for microbial fuel cell applications".SCIENTIFIC REPORTS 6.OCT(2016):35252.
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