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Thermochemical processing of fuels involving the use of molecular oxygen
Guo, Hongfan1; Cheng, Qiuxiang1; Jin, Ze1; Wang, Dan1; Xu, Guangwen2; Liu, Yunyi1
2016
发表期刊RSC ADVANCES
ISSN2046-2069
卷号6期号:104页码:102231-102248
摘要

In a high-temperature (e.g., 1000 degrees C) atmosphere containing combustibles, it is naturally thought that air/O-2 should be kept away for fear of combustion and explosion. However, during thermochemical processing (TCP) of carbonaceous fuels (CFs) it's actually not that simple. TCP, the process for recovering CFs or converting problematic CFs into preferred ones, is a key technology for efficiently and relatively cleanly utilizing various CFs that supply the majority of the worldwide energy demand. However, TCP is often subject to some obstacles (e.g., high energy input and thermodynamic constraint). This review on extensive literature demonstrates that not only does introducing a controlled amount of O-2 (i.e., molecular oxygen) into TCP overcome its many obstacles, but also this O-2-assisted strategy is applicable to all of the main CFs currently known. Despite such a wide applicability to CFs, there lacks a comprehensive consideration of various aerobic TCP processes for understanding the O-2-assisted strategy as a kind of universal TCP technology for CFs. In this review, we for the first time summarize and discuss the use of O-2 in various TCP processes for all of the main CFs. We hope that this review can inspire more consideration of the various aerobic TCP processes so that these extremely complex processes can be communicated or consulted from each other's experience/research findings in order to enlighten, guide or promote their respective development.

文章类型Review
WOS标题词Science & Technology ; Physical Sciences
DOI10.1039/c6ra18616e
收录类别SCI
语种英语
关键词[WOS]IN-SITU COMBUSTION ; UNDERGROUND COAL-GASIFICATION ; SYNTHESIS GAS-PRODUCTION ; CHEMICAL-LOOPING COMBUSTION ; METHANOL CATALYTIC CYCLE ; C-H ACTIVATION ; PARTIAL OXIDATION ; OIL-SHALE ; BIOMASS GASIFICATION ; HYDROGEN-PRODUCTION
WOS研究方向Chemistry
WOS类目Chemistry, Multidisciplinary
项目资助者Program for Liaoning Innovative Research Team in University (LNIRT)(LT2013010) ; Education Administration of Liaoning Province(L2014161) ; State Key Laboratory of Chemical Resource Engineering(CRE-2015-C-109) ; National Natural Science Foundation of China(21403143)
WOS记录号WOS:000387621700060
引用统计
被引频次:2[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/21838
专题多相复杂系统国家重点实验室
作者单位1.Shenyang Univ Chem Technol, Coll Chem Engn, Key Lab Appl Technol Chem Engn Liaoning Prov, Shenyang 110142, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
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GB/T 7714
Guo, Hongfan,Cheng, Qiuxiang,Jin, Ze,et al. Thermochemical processing of fuels involving the use of molecular oxygen[J]. RSC ADVANCES,2016,6(104):102231-102248.
APA Guo, Hongfan,Cheng, Qiuxiang,Jin, Ze,Wang, Dan,Xu, Guangwen,&Liu, Yunyi.(2016).Thermochemical processing of fuels involving the use of molecular oxygen.RSC ADVANCES,6(104),102231-102248.
MLA Guo, Hongfan,et al."Thermochemical processing of fuels involving the use of molecular oxygen".RSC ADVANCES 6.104(2016):102231-102248.
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