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In Situ Catalytic Pyrolysis of Low-Rank Coal for the Conversion of Heavy Oils into Light Oils
Amin, Muhammad Nadeem; Li, Yi; Lu, Xingmei
2017
发表期刊ADVANCES IN MATERIALS SCIENCE AND ENGINEERING
ISSN1687-8434
期号2017页码:5612852
摘要

Lighter tars are largely useful in chemical industries but their quantity is quite little. Catalytic cracking is applied to improve the yield of light tars during pyrolysis. Consequently, in situ upgrading technique through a MoS2 catalyst has been explored in this research work. MoS2 catalyst is useful for the conversion of high energy cost into low energy cost. The variations in coal pyrolysis tar without and with catalyst were determined. Meanwhile, the obtained tar was analyzed using simulated distillation gas chromatograph and Elemental Analyzer. Consequently, the catalyst reduced the pitch contents and increased the fraction of light tar from 50 to 60 wt.% in coal pyrolysis tar. MoS2 catalyst increased the liquid yield from 18 to 33 ( wt.%, db) and decreased gas yield from 27 to 12 ( wt.%, db) compared to coal without catalyst. Moreover, it increased H content and hydrogen-to-carbon ratio by 7.9 and 3.3%, respectively, and reduced the contents of nitrogen, sulphur, and oxygen elements by 8.1%, 15.2%, and 23.9%, respectively, in their produced tars compared to coal without catalyst.

文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1155/2017/5612852
收录类别SCI
语种英语
关键词[WOS]BED REACTOR ; MULTISTAGE HYDROPYROLYSIS ; BROWN-COAL ; TAR ; LIGNITE ; HYDROGENATION ; MICROWAVE ; PRODUCTS ; ZEOLITE ; YIELD
WOS研究方向Materials Science
WOS类目Materials Science, Multidisciplinary
项目资助者Beijing Natural Science Foundation(3142020) ; Strategic Priority Research Program of CAS(XDA07010300) ; CAS Province Cooperation Program(2014JZ0012) ; National Major Instrumentation Development(2011YQ12003907)
WOS记录号WOS:000394135100001
引用统计
被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/21950
专题多相复杂系统国家重点实验室
作者单位Chinese Acad Sci, Inst Proc Engn, Beijing Key Lab Ion Liquids Clean Proc, Key Lab Green Proc & Engn,State Key Lab Multiphas, Beijing 100190, Peoples R China
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Amin, Muhammad Nadeem,Li, Yi,Lu, Xingmei. In Situ Catalytic Pyrolysis of Low-Rank Coal for the Conversion of Heavy Oils into Light Oils[J]. ADVANCES IN MATERIALS SCIENCE AND ENGINEERING,2017(2017):5612852.
APA Amin, Muhammad Nadeem,Li, Yi,&Lu, Xingmei.(2017).In Situ Catalytic Pyrolysis of Low-Rank Coal for the Conversion of Heavy Oils into Light Oils.ADVANCES IN MATERIALS SCIENCE AND ENGINEERING(2017),5612852.
MLA Amin, Muhammad Nadeem,et al."In Situ Catalytic Pyrolysis of Low-Rank Coal for the Conversion of Heavy Oils into Light Oils".ADVANCES IN MATERIALS SCIENCE AND ENGINEERING .2017(2017):5612852.
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