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Kinetic Evaluation of Hydrodesulfurization and Hydrodenitrogenation Reactions via a Lumped Model
Yang, Yiqian1,2,3; Dai, Fei2,3; Li, Chunshan2,3,4; Xiang, Shuguang1; Yaseen, Muhammad2,3; Zhang, Suojiang2,3
2017-05-01
Source PublicationENERGY & FUELS
ISSN0887-0624
Volume31Issue:5Pages:5491-5497
Abstract

Multi-lump kinetic models for model compounds representative of various sulfur (5) and nitrogen (N) compounds in coker gas oil (CGO) were developed to describe CGO hydrodesulfurization (HDS) and hydrodenitrogenation (HDN) processes, respectively. Model parameters were obtained from fitting of operating data. Validation results revealed that models could predict contents of S and N in products accurately, and hydrogen consumption of HDS and HDN can be estimated. The effects of the temperature, hydrogen/oil ratio, and pressure on the reaction performance were also investigated.

SubtypeArticle
WOS HeadingsScience & Technology ; Technology
DOI10.1021/acs.energyfuels.7b00496
Indexed BySCI
Language英语
WOS KeywordCoker Gas Oil ; Coal-tar Hydrogenation ; Shale Oil ; Nimo/al2o3 Catalyst ; Clean Fuel ; Reactor
WOS Research AreaEnergy & Fuels ; Engineering
WOS SubjectEnergy & Fuels ; Engineering, Chemical
Funding OrganizationNational Science Fund for Excellent Young Scholars(21422607) ; National Natural Science Funds(21576261) ; National Key Research and Development Program(2016YFB0601303) ; Innovation Fund of PetroChina(2015D-5006-0406)
WOS IDWOS:000402023600095
Citation statistics
Cited Times:4[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/22645
Collection多相复杂系统国家重点实验室
Affiliation1.Qingdao Univ Sci & Technol, Hitech Inst Petr & Chem Ind, Qingdao 266042, Shandong, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, Natl Key Lab Clean & Efficient Coking Technol, Beijing 100190, Peoples R China
4.Univ Chinese Acad Sci, Sch Chem & Chem Engn, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Yang, Yiqian,Dai, Fei,Li, Chunshan,et al. Kinetic Evaluation of Hydrodesulfurization and Hydrodenitrogenation Reactions via a Lumped Model[J]. ENERGY & FUELS,2017,31(5):5491-5497.
APA Yang, Yiqian,Dai, Fei,Li, Chunshan,Xiang, Shuguang,Yaseen, Muhammad,&Zhang, Suojiang.(2017).Kinetic Evaluation of Hydrodesulfurization and Hydrodenitrogenation Reactions via a Lumped Model.ENERGY & FUELS,31(5),5491-5497.
MLA Yang, Yiqian,et al."Kinetic Evaluation of Hydrodesulfurization and Hydrodenitrogenation Reactions via a Lumped Model".ENERGY & FUELS 31.5(2017):5491-5497.
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