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题名:
Production of Bio-Based Gasoline by Noble-Metal-Catalyzed Hydrodeoxygenation of alpha-Angelica Lactone Derived Di/Trimers
作者: Ayodele, Olubunmi O.1,2,3; Dawodu, Folasegun A.2; Yan, Dongxia1; Dong, Huixian1; Xin, Jiayu1; Zhang, Suojiang1
刊名: CHEMISTRYSELECT
出版日期: 2017-05-23
卷号: 2, 期号:15, 页码:4219-4225
关键词: Angelica lactone ; biomass ; C-C coupling ; catalysts ; hydrodeoxygenation
收录类别: SCI
WOS记录号: WOS:000402286000008
DOI: 10.1002/slct.201700451
文章类型: Article
英文摘要: Conversion of biomass into a suitable fuel involves series of chemical transformation including C-C coupling and hydrodeoxygenation reactions. Here, we have employed coupling reaction to a biomass-derived angelica lactone in the presence of mild alkaline catalysts, K2CO3 to obtain dimers and trimers in appropriate quantities. Hydrodeoxygenation of these molecules over carbon-supported noble metal catalysts was performed. Subsequently, the effect of operating parameters such as hydrogen pressure, temperature and reaction time on the hydrodeoxygenation of di/trimers were fully optimized and liquids suitable for gasoline application were obtained. This process has the potential of scale-up since the raw materials can easily be obtained from freely available biomass and the technology involved in carbon-carbon coupling and hydrodeoxygenation is well known.
WOS标题词: Science & Technology ; Physical Sciences
类目[WOS]: Chemistry, Multidisciplinary
研究领域[WOS]: Chemistry
关键词[WOS]: HIGH-QUALITY DIESEL ; TRANSPORTATION FUELS ; GAMMA-VALEROLACTONE ; CARBON-DIOXIDE ; BIOMASS ; LIQUID ; HYDROCARBONS ; CONVERSION ; HYDROGEN ; ALKANES
项目资助者: International S&T Cooperation Program of China(2014DFA61670) ; National Natural Science Foundation of China(21576269 ; BIC, Chinese Academy of Sciences(GJHZ201306) ; World Academy of Sciences (TWAS) ; Chinese Academy of Sciences (CAS) ; 21276260 ; 21210006)
语种: 英语
ISSN号: 2365-6549
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.ipe.ac.cn/handle/122111/22658
Appears in Collections:多相复杂系统国家重点实验室_期刊论文

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作者单位: 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Key Lab Green Proc & Engn, Beijing 100190, Peoples R China
2.Univ Ibadan, Dept Ind Chem, Ibadan, Oyo State, Nigeria
3.Forestry Res Inst Nigeria, Dept Forest Prod Dev & Utilizat, Ibadan, Oyo State, Nigeria

Recommended Citation:
Ayodele, Olubunmi O.,Dawodu, Folasegun A.,Yan, Dongxia,et al. Production of Bio-Based Gasoline by Noble-Metal-Catalyzed Hydrodeoxygenation of alpha-Angelica Lactone Derived Di/Trimers[J]. CHEMISTRYSELECT,2017,2(15):4219-4225.
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