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Production of Bio-Based Gasoline by Noble-Metal-Catalyzed Hydrodeoxygenation of alpha-Angelica Lactone Derived Di/Trimers
Ayodele, Olubunmi O.1,2,3; Dawodu, Folasegun A.2; Yan, Dongxia1; Dong, Huixian1; Xin, Jiayu1; Zhang, Suojiang1
2017-05-23
发表期刊CHEMISTRYSELECT
ISSN2365-6549
卷号2期号:15页码:4219-4225
摘要Conversion of biomass into a suitable fuel involves series of chemical transformation including C-C coupling and hydrodeoxygenation reactions. Here, we have employed coupling reaction to a biomass-derived angelica lactone in the presence of mild alkaline catalysts, K2CO3 to obtain dimers and trimers in appropriate quantities. Hydrodeoxygenation of these molecules over carbon-supported noble metal catalysts was performed. Subsequently, the effect of operating parameters such as hydrogen pressure, temperature and reaction time on the hydrodeoxygenation of di/trimers were fully optimized and liquids suitable for gasoline application were obtained. This process has the potential of scale-up since the raw materials can easily be obtained from freely available biomass and the technology involved in carbon-carbon coupling and hydrodeoxygenation is well known.
关键词Angelica Lactone Biomass C-c Coupling Catalysts Hydrodeoxygenation
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
DOI10.1002/slct.201700451
收录类别SCI
语种英语
关键词[WOS]HIGH-QUALITY DIESEL ; TRANSPORTATION FUELS ; GAMMA-VALEROLACTONE ; CARBON-DIOXIDE ; BIOMASS ; LIQUID ; HYDROCARBONS ; CONVERSION ; HYDROGEN ; ALKANES
WOS研究方向Chemistry
WOS类目Chemistry, Multidisciplinary
项目资助者International S&T Cooperation Program of China(2014DFA61670) ; National Natural Science Foundation of China(21576269 ; BIC, Chinese Academy of Sciences(GJHZ201306) ; World Academy of Sciences (TWAS) ; Chinese Academy of Sciences (CAS) ; 21276260 ; 21210006)
WOS记录号WOS:000402286000008
引用统计
被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/22658
专题多相复杂系统国家重点实验室
作者单位1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Key Lab Green Proc & Engn, Beijing 100190, Peoples R China
2.Univ Ibadan, Dept Ind Chem, Ibadan, Oyo State, Nigeria
3.Forestry Res Inst Nigeria, Dept Forest Prod Dev & Utilizat, Ibadan, Oyo State, Nigeria
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Ayodele, Olubunmi O.,Dawodu, Folasegun A.,Yan, Dongxia,et al. Production of Bio-Based Gasoline by Noble-Metal-Catalyzed Hydrodeoxygenation of alpha-Angelica Lactone Derived Di/Trimers[J]. CHEMISTRYSELECT,2017,2(15):4219-4225.
APA Ayodele, Olubunmi O.,Dawodu, Folasegun A.,Yan, Dongxia,Dong, Huixian,Xin, Jiayu,&Zhang, Suojiang.(2017).Production of Bio-Based Gasoline by Noble-Metal-Catalyzed Hydrodeoxygenation of alpha-Angelica Lactone Derived Di/Trimers.CHEMISTRYSELECT,2(15),4219-4225.
MLA Ayodele, Olubunmi O.,et al."Production of Bio-Based Gasoline by Noble-Metal-Catalyzed Hydrodeoxygenation of alpha-Angelica Lactone Derived Di/Trimers".CHEMISTRYSELECT 2.15(2017):4219-4225.
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