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Preparation of carbon-Ni/MgO-Al2O3 composite catalysts for CO2 reforming of methane
Jin, Lijun1,2; Xie, Tong1; Ma, Bingxue1; Li, Yang1; Hu, Haoquan1
2017-02-23
发表期刊INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
ISSN0360-3199
卷号42期号:8页码:5047-5055
摘要Carbon-Ni/MgO-Al2O3 composite catalysts were prepared using sucrose as carbon precursor and [Ni,Mg,Al]-layered double hydroxide (LDH) as Ni-based catalyst precursor by impregnation method, characterized and used for CO2 reforming of CH4. The results showed that pretreated temperature of LDH, carbonization temperature of composite catalyst precursors and the sucrose/layered double oxide (LDO) mass ratio have obvious effect on the structure and catalytic performances of the resultant composite catalysts. The incorporation of carbon into Ni-based catalyst results in the increase of specific surface area, anti-coke ability, inhibition of Ni particle growth and catalytic stability, but a little decrease in initial activities of catalysts owing to low catalytic activity of the carbon. At an appropriate condition with LDH pretreated temperature of 350 degrees C, carbonization temperature of 800 degrees C and sucrose/LDO ratio of 1.2, the resultant composite catalyst exhibits the best activity and stability. (C) 2016 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
关键词Co2 Reforming Of Ch4 Ni/mgo-al2o3 Sucrose Composite Catalyst Layered Double Hydroxide
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.ijhydene.2016.11.130
收录类别SCI
语种英语
关键词[WOS]LAYERED DOUBLE HYDROXIDES ; CARBON-DIOXIDE ; SYNTHESIS GAS ; HYDROGEN ; CH4 ; NI ; DECOMPOSITION ; PRECURSORS ; PERFORMANCE ; SYNGAS
WOS研究方向Chemistry ; Electrochemistry ; Energy & Fuels
WOS类目Chemistry, Physical ; Electrochemistry ; Energy & Fuels
项目资助者Coal-based Low Hydrocarbons by NSFC(U1510101) ; Shanxi Provincial Government(U1510101) ; National Key Research and Development Program of China(2016YFB0600301) ; NSFC(U1503194) ; Xinjiang Provincial Government(U1503194) ; Liaoning Province Education Administration Fund(L2013028) ; State Key Laboratory of Multiphase Complex Systems(MPCS-2014-D-07) ; Fundamental Research Funds for the Central Universities(DUT15LAB09)
WOS记录号WOS:000403852600032
引用统计
被引频次:5[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/22721
专题多相复杂系统国家重点实验室
作者单位1.Dalian Univ Technol, Sch Chem Engn, Inst Coal Chem Engn, State Key Lab Fine Chem, Dalian 116024, Liaoning, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
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GB/T 7714
Jin, Lijun,Xie, Tong,Ma, Bingxue,et al. Preparation of carbon-Ni/MgO-Al2O3 composite catalysts for CO2 reforming of methane[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2017,42(8):5047-5055.
APA Jin, Lijun,Xie, Tong,Ma, Bingxue,Li, Yang,&Hu, Haoquan.(2017).Preparation of carbon-Ni/MgO-Al2O3 composite catalysts for CO2 reforming of methane.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,42(8),5047-5055.
MLA Jin, Lijun,et al."Preparation of carbon-Ni/MgO-Al2O3 composite catalysts for CO2 reforming of methane".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 42.8(2017):5047-5055.
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