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Catalyst Grading Optimization and Kinetic Simulation of the Shale Oil Hydrotreating Process
Wang, Hongyan1,2; Dai, Fei1,2; Yang, Yiqian1,2; Li, Zengxi3; Li, Chunshan1,2; Zhang, Suojiang1,2
2017-04-01
发表期刊ENERGY & FUELS
ISSN0887-0624
卷号31期号:4页码:4353-4360
摘要The shale oil hydrogenation experiments were conducted on a fixed-bed reactor with grading of a hydrogenating protective (HP) catalyst, hydrofining (HF) catalyst, and hydrocracking (HC) catalyst. The effects of the reaction temperature and liquid hourly space velocity (LHSV) on product distribution of shale oil hydrotreating were investigated. Three kinds of lumping kinetic models for,hydrodearomatization (HDA), hydrodesulfurization (HDS), and hydrodenitrogenation (HDN) were first established and applied in this process. The predicted reactive features and optimized operating conditions for HDS, HDN, and HDA agreed well with experimental results at different catalyst grading ratios, with a relative error of less than 3.8%. In accordance with operating conditions, the model can also be applied in catalyst grading scale calculation, which enhances the theory of shale oil hydro-upgrading application.
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1021/acs.energyfuels.6b02720
收录类别SCI
语种英语
关键词[WOS]COAL-TAR HYDROGENATION ; TRICKLE-BED REACTOR ; DISTILLATION FRACTIONS ; HYDRODESULFURIZATION PROCESS ; NITROGEN-COMPOUNDS ; DIESEL FRACTION ; LIGHT MAZUTE ; CLEAN FUEL ; YIELD ; HYDRODENITROGENATION
WOS研究方向Energy & Fuels ; Engineering
WOS类目Energy & Fuels ; Engineering, Chemical
项目资助者National Basic Research Program of China (973 Program)(2014CB744306) ; National Science Fund for Excellent Young Scholars(21422607) ; General Program of National Natural Science Foundation of China(21576261) ; National Natural Science Foundation of China(PRIKY15013 ; 2015D-5006-0406)
WOS记录号WOS:000400039800108
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被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/22830
专题多相复杂系统国家重点实验室
作者单位1.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Natl Key Lab Clean & Efficient Coking Technol, Inst Proc Engn, Beijing 100190, Peoples R China
3.Univ Chinese Acad Sci, Coll Chem & Chem Engn, Beijing 100049, Peoples R China
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GB/T 7714
Wang, Hongyan,Dai, Fei,Yang, Yiqian,et al. Catalyst Grading Optimization and Kinetic Simulation of the Shale Oil Hydrotreating Process[J]. ENERGY & FUELS,2017,31(4):4353-4360.
APA Wang, Hongyan,Dai, Fei,Yang, Yiqian,Li, Zengxi,Li, Chunshan,&Zhang, Suojiang.(2017).Catalyst Grading Optimization and Kinetic Simulation of the Shale Oil Hydrotreating Process.ENERGY & FUELS,31(4),4353-4360.
MLA Wang, Hongyan,et al."Catalyst Grading Optimization and Kinetic Simulation of the Shale Oil Hydrotreating Process".ENERGY & FUELS 31.4(2017):4353-4360.
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