CAS OpenIR  > 多相复杂系统国家重点实验室
In Situ Electrochemistry of Rechargeable Battery Materials: Status Report and Perspectives
Yang, Yijun1; Liu, Xizheng2; Dai, Zhonghua5; Yuan, Fangli6; Bando, Yoshio7,8; Golberg, Dmitri7,9; Wang, Xi1,3,4
2017-08-18
Source PublicationADVANCED MATERIALS
ISSN0935-9648
Volume29Issue:31
Abstract

The development of rechargeable batteries with high performance is considered to be a feasible way to satisfy the increasing needs of electric vehicles and portable devices. It is of vital importance to design electrodes with high electrochemical performance and to understand the nature of the electrode/electrolyte interfaces during battery operation, which allows a direct observation of the complicated chemical and physical processes within the electrodes and electrolyte, and thus provides real-time information for further design and optimization of the battery performance. Here, the recent progress in in situ techniques employed for the investigations of material structural evolutions is described, including characterization using neutrons, X-ray diffraction, and nuclear magnetic resonance. In situ techniques utilized for in-depth uncovering the electrode/electrolyte phase/interface change mechanisms are then highlighted, including transmission electron microscopy, atomic force microscopy, X-ray spectroscopy, and Raman spectroscopy. The real-time monitoring of lithium dendrite growth and in situ detection of gas evolution during charge/discharge processes are also discussed. Finally, the major challenges and opportunities of in situ characterization techniques are outlined toward new developments of rechargeable batteries, including innovation in the design of compatible in situ cells, applications of dynamic analysis, and in situ electrochemistry under multi-stimuli. A clear and in-depth understanding of in situ technique applications and the mechanisms of structural evolutions, surface/interface changes, and gas generations within rechargeable batteries is given here.

KeywordIn Situ Electrochemical Rechargeable Batteries Structure Evolution Surface/interface Changes
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1002/adma.201606922
Indexed BySCI
Language英语
WOS KeywordLithium-ion Batteries ; Atomic-force Microscopy ; X-ray-diffraction ; Solid-electrolyte Interphase ; Carbonate-based Electrolytes ; Silicon Nanowire Anodes ; Li-s Batteries ; Graphite-electrodes ; Neutron-diffraction ; Amorphous-silicon
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS SubjectChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
Funding OrganizationBeijing JiaoTong University ; National Natural Science Foundation of China(21603162 ; Australian Research Council (ARC) ; 11535003)
WOS IDWOS:000407565700002
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/23176
Collection多相复杂系统国家重点实验室
Affiliation1.Beijing Jiaotong Univ, Sch Sci, Minist Educ, Key Lab Luminescence & Opt Informat, Beijing 100044, Peoples R China
2.Tianjin Univ Technol, Sch Mat Sci & Engn, Inst New Energy Mat & Low Carbon Technol, Tianjin Key Lab Adv Funct Porous Mat, Tianjin 300384, Peoples R China
3.Tianjin Univ, Dept Chem, Tianjin Key Lab Mol Optoelect Sci, Tianjin 3003072, Peoples R China
4.Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 3003072, Peoples R China
5.Xian Technol Univ, Lab Thin Film Tech & Opt Test, Xian 710032, Shaanxi, Peoples R China
6.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Zhongguancun Beiertiao 1 Hao, Beijing 100190, Peoples R China
7.Natl Inst Mat Sci, World Premier Int Ctr Mat Nanoarchitecton, WPI MANA, Namiki 1-1, Tsukuba, Ibaraki 3050044, Japan
8.Univ Wollongong, AIIM, Squires Way, North Wollongong, NSW 2500, Australia
9.Queensland Univ Technol, Sci & Engn Fac, 2 George St, Brisbane, Qld 4000, Australia
Recommended Citation
GB/T 7714
Yang, Yijun,Liu, Xizheng,Dai, Zhonghua,et al. In Situ Electrochemistry of Rechargeable Battery Materials: Status Report and Perspectives[J]. ADVANCED MATERIALS,2017,29(31).
APA Yang, Yijun.,Liu, Xizheng.,Dai, Zhonghua.,Yuan, Fangli.,Bando, Yoshio.,...&Wang, Xi.(2017).In Situ Electrochemistry of Rechargeable Battery Materials: Status Report and Perspectives.ADVANCED MATERIALS,29(31).
MLA Yang, Yijun,et al."In Situ Electrochemistry of Rechargeable Battery Materials: Status Report and Perspectives".ADVANCED MATERIALS 29.31(2017).
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