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Ionic-Liquid-Based CO2 Capture Systems: Structure, Interaction and Process
Zeng, Shaojuan1; Zhang, Xianping1,2; Bai, Lu1; Zhang, Xiaochun1; Wang, Hui1; Wang, Jianji3; Bao, Di1,2; Li, Mengdie1,2; Liu, Xinyan1,2; Zhang, Suojiang1
Source PublicationCHEMICAL REVIEWS

The inherent structure tunability, good affinity with CO2, and nonvolatility of ionic liquids (ILs) drive their exploration and exploitation in CO2 separation field, and has attracted remarkable interest from both industries and academia. The aim of this Review is to give a detailed overview on the recent advances on IL-based materials, including pure ILs, IL-based solvents, and IL-based membranes for CO2 capture and separation from the viewpoint of molecule to engineering. The effects of anions, cations and functional groups on CO2 solubility and selectivity of ILs, as well as the studies on degradability of ILs are reviewed, and the recent developments on functionalized ILs, IL-based solvents, and IL-based membranes are also discussed. CO2 separation mechanism with IL-based solvents and IL-based membranes are explained by combining molecular simulation and experimental characterization. Taking into consideration of the applications and industrialization, the recent achievements and developments on the transport properties of IL fluids and the process design of IL-based processes are highlighted. Finally, the future research challenges and perspectives of the commercialization of CO2 capture and separation with IL-based materials are posed.

WOS HeadingsScience & Technology ; Physical Sciences
Indexed BySCI
WOS KeywordCarbon-dioxide Capture ; Pressure Phase-behavior ; Gas Separation Performance ; Mixed-matrix Membranes ; Methyldiethanolamine Aqueous-solution ; Facilitated Transport Membranes ; Molecular-dynamics Simulation ; Co2-binding Organic Liquids ; Activated Mdea Solutions ; Of-the-art
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationNational Natural Science Foundation of China(21425625 ; Capital Science and Technology Leading Talent Training Project(1j201710) ; 21506219 ; U1662122 ; 51674234 ; 21606233 ; 21676271)
WOS IDWOS:000406649300004
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Document Type期刊论文
Affiliation1.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, Key Lab Green Proc & Engn, State Key Lab Multiphase Complex Syst,Inst Proc E, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Coll Chem & Engn, Beijing 100049, Peoples R China
3.Henan Normal Univ, Sch Chem & Environm Sci, Xinxiang 453007, Henan, Peoples R China
Recommended Citation
GB/T 7714
Zeng, Shaojuan,Zhang, Xianping,Bai, Lu,et al. Ionic-Liquid-Based CO2 Capture Systems: Structure, Interaction and Process[J]. CHEMICAL REVIEWS,2017,117(14):9625-9673.
APA Zeng, Shaojuan.,Zhang, Xianping.,Bai, Lu.,Zhang, Xiaochun.,Wang, Hui.,...&Zhang, Suojiang.(2017).Ionic-Liquid-Based CO2 Capture Systems: Structure, Interaction and Process.CHEMICAL REVIEWS,117(14),9625-9673.
MLA Zeng, Shaojuan,et al."Ionic-Liquid-Based CO2 Capture Systems: Structure, Interaction and Process".CHEMICAL REVIEWS 117.14(2017):9625-9673.
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