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Pinecone biomass-derived hard carbon anodes for high-performance sodium-ion batteries
Zhang, Tao1,2; Mao, Jing1,2; Liu, Xiaolin1; Xuan, Minjie1,2; Bi, Kai1; Zhang, Xiao Li1,2; Hu, Junhua1,2; Fan, Jiajie1,2; Chen, Shimou3; Shao, Guosheng1,2
2017
Source PublicationRSC ADVANCES
ISSN2046-2069
Volume7Issue:66Pages:41504-41511
AbstractHard-carbon is considered as one of the most promising anode materials for sodium-ion batteries (SIBs). Now it is imperative to develop a proper preparation method to obtain hard carbon anode particles with high initial coulombic efficiency and good cycling performance. In this paper, we have successfully prepared high performance hard carbon anodes, by selecting abundant and low-cost pinecones as biomass precursor and optimizing the preparation parameters of pinecone-derived hard carbon (PHC). The microstructure of PHC is studied by X-ray diffraction (XRD), Raman spectroscopy, high-resolution transmission electron microscopy (HRTEM) as well as nitrogen adsorption-desorption isotherm methods. The performance of PHC is highly dependent on the carbonization temperature. Increasing carbonization temperature of pinecone precursor can reduce surface area and thus improve the initial coulombic efficiency. Varying carbonization temperature can also adjust the slope and plateau capacity of PHC, and then regulate the energy density and power characteristics of PHC in battery operation. PHC1400 still delivers a capacity of 334 mA h g(-1) after 120 cycles, with a high initial coulombic efficiency of 85.4%. Our results suggest that PHC is a promising anode material for practical large-scale SIB application.
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
DOI10.1039/c7ra07231g
Indexed BySCI
Language英语
WOS KeywordHIGH-CAPACITY ; ENERGY-STORAGE ; GRAPHITE ; NANOCOMPOSITE ; ELECTROLYTE
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationNational Natural Science Foundation of China(U1504521 ; Fundamental Research Program from the Ministry of Science and Technology of China(2014CB931704) ; 51604224)
WOS IDWOS:000409147000024
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/23185
Collection研究所(批量导入)
Affiliation1.Zhengzhou Univ, Sch Mat Sci & Engn, Zhengzhou 450001, Henan, Peoples R China
2.Zhengzhou Univ, State Ctr Int Cooperat Designer Low Carbon & Env, Zhengzhou 450001, Henan, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Tao,Mao, Jing,Liu, Xiaolin,et al. Pinecone biomass-derived hard carbon anodes for high-performance sodium-ion batteries[J]. RSC ADVANCES,2017,7(66):41504-41511.
APA Zhang, Tao.,Mao, Jing.,Liu, Xiaolin.,Xuan, Minjie.,Bi, Kai.,...&Shao, Guosheng.(2017).Pinecone biomass-derived hard carbon anodes for high-performance sodium-ion batteries.RSC ADVANCES,7(66),41504-41511.
MLA Zhang, Tao,et al."Pinecone biomass-derived hard carbon anodes for high-performance sodium-ion batteries".RSC ADVANCES 7.66(2017):41504-41511.
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