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Polycyclic aromatic hydrocarbons on particulate matter emitted during the co-generation of bioenergy and biochar from rice husk
Dunnigan, Lewis1; Morton, Benjamin J.1; van Eyk, Philip J.1; Ashman, Peter J.1; Zhang, Xiangping2; Hall, Philip Anthony3; Kwong, Chi Wai1
2017-11-01
发表期刊BIORESOURCE TECHNOLOGY
ISSN0960-8524
卷号244期号:NOV页码:1015-1023
摘要

The aim of this study was to evaluate the emissions of polycyclic aromatic hydrocarbons (PAHs) bound to the particulate matter (PM) during the combustion of raw pyrolysis volatiles (bio-oil and pyrogas mixture) generated from the pyrolysis of rice husk. Five different raw pyrolysis volatiles were produced at varying pyrolysis temperatures (400-800 degrees C) and subsequently combusted in a laboratory-scale, continuous pyrolysis-combustion facility at 850 degrees C. 15 priority pollutant PAH levels in the resulting biochar, bio-oil, and PM were evaluated. Results showed that combustion of the raw pyrolysis volatiles produced at elevated pyrolysis temperatures resulted in greater concentrations of PM-bound PAHs (119% increase between 400 and 800 degrees C) due to the increased PAH and oxy-aromatic content of the bio-oil fraction. Significantly increased benzo(a) pyrene (BaP) equivalent toxicity of the biochar and PM was observed at elevated pyrolysis temperatures.

关键词Pah Biochar Bioenergy Toxicity Pm
文章类型Article
WOS标题词Science & Technology ; Life Sciences & Biomedicine ; Technology
DOI10.1016/j.biortech.2017.08.091
收录类别SCI
语种英语
关键词[WOS]SEWAGE-SLUDGE ; BIO-OIL ; PYROLYSIS ; COMBUSTION ; TEMPERATURE ; FUEL ; EMISSION ; PAHS ; COAL ; GASIFICATION
WOS研究方向Agriculture ; Biotechnology & Applied Microbiology ; Energy & Fuels
WOS类目Agricultural Engineering ; Biotechnology & Applied Microbiology ; Energy & Fuels
项目资助者Government of South Australia through the Premier's Research and Industry Fund Catalyst Research Grants(CGR72) ; Trevor Prescott Memorial Scholarship
WOS记录号WOS:000410545300125
引用统计
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/23240
专题多相复杂系统国家重点实验室
作者单位1.Univ Adelaide, Sch Chem Engn, Adelaide, SA 5005, Australia
2.Chinese Acad Sci, Inst Proc Engn, Beijing, Peoples R China
3.Univ Adelaide, Sch Phys Sci, Adelaide, SA 5005, Australia
推荐引用方式
GB/T 7714
Dunnigan, Lewis,Morton, Benjamin J.,van Eyk, Philip J.,et al. Polycyclic aromatic hydrocarbons on particulate matter emitted during the co-generation of bioenergy and biochar from rice husk[J]. BIORESOURCE TECHNOLOGY,2017,244(NOV):1015-1023.
APA Dunnigan, Lewis.,Morton, Benjamin J..,van Eyk, Philip J..,Ashman, Peter J..,Zhang, Xiangping.,...&Kwong, Chi Wai.(2017).Polycyclic aromatic hydrocarbons on particulate matter emitted during the co-generation of bioenergy and biochar from rice husk.BIORESOURCE TECHNOLOGY,244(NOV),1015-1023.
MLA Dunnigan, Lewis,et al."Polycyclic aromatic hydrocarbons on particulate matter emitted during the co-generation of bioenergy and biochar from rice husk".BIORESOURCE TECHNOLOGY 244.NOV(2017):1015-1023.
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