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In Situ Self-Assembly-Generated 3D Hierarchical Co3O4 Micro/Nanomaterial Series: Selective Synthesis, Morphological Control, and Energy Applications
Miao, Qingqing; Zhang, Suojiang
2017-12-20
发表期刊ACS APPLIED MATERIALS & INTERFACES
ISSN1944-8244
卷号9期号:50页码:44199-44213
摘要

A simple in situ self-assembly selective synthetic strategy for onestep controllable formation of various three-dimensional (3D) hierarchical Co3O4 micro/nanomaterials with peculiar morphologies, uniform size, and high quality is successfully developed. The Morphological control and related impact factors are investigated and clarified in detail. The results further clarify the corresponding mechanisms on the reaction process, product generation, and calcining process as well as the formation of specific morphologies. Furthermore, the superior catalytic properties of these materials are confirmed by two typical Co-based energy applications on the decomposition of an important solid rocket propellant, ammonium perchlorate (AP), and dye-sensitized solar cells (DSSCs). The addition of Co3O4 materials to AP obviously decreases the decomposition temperatures by about 118-140 degrees C and increases the exothermic heat to a great extent. As the substituted counter electrodes of DSSCs, the 3D hierarchical Co3O4 materials exhibit attractive photovoltaic performances. These findings provide a facile and: effective way for designing new types of 3D hierarchical materials toward high catalytic activity for energy devices.

关键词In Situ 3d Hierarchical Co3o4 Micro/nanomaterials Superior Catalytic Properties Ammonium Perchlorate Dye-sensitized Solar Cells
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1021/acsami.7b14543
收录类别SCI
语种英语
关键词[WOS]Sensitized Solar-cells ; Lithium-ion Batteries ; Chemical-vapor-deposition ; Electrochemical Performance ; Nanowire Arrays ; Water Oxidation ; Storage Properties ; Mesoporous Co3o4 ; High-efficiency ; Hollow Spheres
WOS研究方向Science & Technology - Other Topics ; Materials Science
WOS类目Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
项目资助者National Natural Science Foundation of China(51203161 ; Key Laboratory of Green Process and Engineering, Chinese Academy of Sciences ; 21576264 ; 21436010 ; 91434203)
WOS记录号WOS:000418783700090
引用统计
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/23480
专题研究所(批量导入)
通讯作者Zhang, Suojiang
作者单位Chinese Acad Sci, State Key Lab Multiphase Complex Syst, Beijing Key Lab Ion Liquids Clean Proc, Key Lab Green Proc & Engn,Inst Proc Engn, 1 Zhongguancun North Second St, Beijing 100190, Peoples R China
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GB/T 7714
Miao, Qingqing,Zhang, Suojiang. In Situ Self-Assembly-Generated 3D Hierarchical Co3O4 Micro/Nanomaterial Series: Selective Synthesis, Morphological Control, and Energy Applications[J]. ACS APPLIED MATERIALS & INTERFACES,2017,9(50):44199-44213.
APA Miao, Qingqing,&Zhang, Suojiang.(2017).In Situ Self-Assembly-Generated 3D Hierarchical Co3O4 Micro/Nanomaterial Series: Selective Synthesis, Morphological Control, and Energy Applications.ACS APPLIED MATERIALS & INTERFACES,9(50),44199-44213.
MLA Miao, Qingqing,et al."In Situ Self-Assembly-Generated 3D Hierarchical Co3O4 Micro/Nanomaterial Series: Selective Synthesis, Morphological Control, and Energy Applications".ACS APPLIED MATERIALS & INTERFACES 9.50(2017):44199-44213.
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