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Fischer-Trospch synthesis using iron-based catalyst in a microchannel reactor: Hybrid lump kinetic with ANNs/RSM | |
Sun, Yong1; Yang, Gang2; Zhang, Lian3; Sun, Zhi4 | |
2017-12-01 | |
Source Publication | CHEMICAL ENGINEERING AND PROCESSING
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ISSN | 0255-2701 |
Volume | 122Issue:00Pages:181-189 |
Abstract | A hybrid methodology of using lump kinetic and of AANs (Artificial Neuron Networks)/RSM (Response Surface Methodology) was investigated for modeling Fischer-Tropsch (FT) synthesis in a microchannel reactor using iron-based catalyst in this work. This robust and cost-effective methodology was reliable to extensively analyze the effect of operating conditions including TOS (time on stream), partial pressures of different gases in reaction system (H-2, CO, CO2 and H2O) on CO disappearance rate. With experimental data as training data set using ANNs and Box-Behnken design as design of experiment, the setup model was able to present good results in nonlinear noisy processes with significant changes of operational parameters in experimental design plan. The proposed hybrid methodology was able to provide comprehensive information such as reaction mechanism, the multiple combined effects on the studied response, and significance of process parameters during FT synthesis using iron-based catalyst in microchannel reactor. |
Keyword | Lump Kinetics Anns/rsm Iron-based Catalyst Microchannel Reactor |
Subtype | Article |
WOS Headings | Science & Technology ; Technology |
DOI | 10.1016/j.cep.2017.10.005 |
Indexed By | SCI |
Language | 英语 |
WOS Keyword | Artificial Neural-networks ; Tropsch Synthesis ; Supported Cobalt ; Liquid Hydrocarbons ; Nsga-ii ; Optimization ; Syngas ; Carbon ; Model ; Nanoparticles |
WOS Research Area | Energy & Fuels ; Engineering |
WOS Subject | Energy & Fuels ; Engineering, Chemical |
Funding Organization | Anpeng high-tech energy-resources Co. Ltd |
WOS ID | WOS:000418211800017 |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.ipe.ac.cn/handle/122111/23494 |
Collection | 研究所(批量导入) |
Corresponding Author | Sun, Yong; Sun, Zhi |
Affiliation | 1.Edith Cowan Univ, Sch Engn, 270 Joondalup Dr, Joondalup, WA 6027, Australia 2.Anpeng High Tech Energy Corp, Beijing, Peoples R China 3.Monash Univ, Dept Chem Engn, Clayton, Vic 3800, Australia 4.Chinese Acad Sci, Inst Proc Engn, Natl Engn Lab Hydromet Cleaner Prod Technol, Beijing 100190, Peoples R China |
Recommended Citation GB/T 7714 | Sun, Yong,Yang, Gang,Zhang, Lian,et al. Fischer-Trospch synthesis using iron-based catalyst in a microchannel reactor: Hybrid lump kinetic with ANNs/RSM[J]. CHEMICAL ENGINEERING AND PROCESSING,2017,122(00):181-189. |
APA | Sun, Yong,Yang, Gang,Zhang, Lian,&Sun, Zhi.(2017).Fischer-Trospch synthesis using iron-based catalyst in a microchannel reactor: Hybrid lump kinetic with ANNs/RSM.CHEMICAL ENGINEERING AND PROCESSING,122(00),181-189. |
MLA | Sun, Yong,et al."Fischer-Trospch synthesis using iron-based catalyst in a microchannel reactor: Hybrid lump kinetic with ANNs/RSM".CHEMICAL ENGINEERING AND PROCESSING 122.00(2017):181-189. |
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File Name/Size | DocType | Version | Access | License | ||
Fischer-Trospch synt(1715KB) | 期刊论文 | 出版稿 | 限制开放 | CC BY-NC-SA | Application Full Text |
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