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Fischer-Trospch synthesis using iron-based catalyst in a microchannel reactor: Hybrid lump kinetic with ANNs/RSM
Sun, Yong1; Yang, Gang2; Zhang, Lian3; Sun, Zhi4
2017-12-01
发表期刊CHEMICAL ENGINEERING AND PROCESSING
ISSN0255-2701
卷号122期号:00页码:181-189
摘要

A hybrid methodology of using lump kinetic and of AANs (Artificial Neuron Networks)/RSM (Response Surface Methodology) was investigated for modeling Fischer-Tropsch (FT) synthesis in a microchannel reactor using iron-based catalyst in this work. This robust and cost-effective methodology was reliable to extensively analyze the effect of operating conditions including TOS (time on stream), partial pressures of different gases in reaction system (H-2, CO, CO2 and H2O) on CO disappearance rate. With experimental data as training data set using ANNs and Box-Behnken design as design of experiment, the setup model was able to present good results in nonlinear noisy processes with significant changes of operational parameters in experimental design plan. The proposed hybrid methodology was able to provide comprehensive information such as reaction mechanism, the multiple combined effects on the studied response, and significance of process parameters during FT synthesis using iron-based catalyst in microchannel reactor.

关键词Lump Kinetics Anns/rsm Iron-based Catalyst Microchannel Reactor
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1016/j.cep.2017.10.005
收录类别SCI
语种英语
关键词[WOS]Artificial Neural-networks ; Tropsch Synthesis ; Supported Cobalt ; Liquid Hydrocarbons ; Nsga-ii ; Optimization ; Syngas ; Carbon ; Model ; Nanoparticles
WOS研究方向Energy & Fuels ; Engineering
WOS类目Energy & Fuels ; Engineering, Chemical
项目资助者Anpeng high-tech energy-resources Co. Ltd
WOS记录号WOS:000418211800017
引用统计
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/23494
专题研究所(批量导入)
通讯作者Sun, Yong; Sun, Zhi
作者单位1.Edith Cowan Univ, Sch Engn, 270 Joondalup Dr, Joondalup, WA 6027, Australia
2.Anpeng High Tech Energy Corp, Beijing, Peoples R China
3.Monash Univ, Dept Chem Engn, Clayton, Vic 3800, Australia
4.Chinese Acad Sci, Inst Proc Engn, Natl Engn Lab Hydromet Cleaner Prod Technol, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Sun, Yong,Yang, Gang,Zhang, Lian,et al. Fischer-Trospch synthesis using iron-based catalyst in a microchannel reactor: Hybrid lump kinetic with ANNs/RSM[J]. CHEMICAL ENGINEERING AND PROCESSING,2017,122(00):181-189.
APA Sun, Yong,Yang, Gang,Zhang, Lian,&Sun, Zhi.(2017).Fischer-Trospch synthesis using iron-based catalyst in a microchannel reactor: Hybrid lump kinetic with ANNs/RSM.CHEMICAL ENGINEERING AND PROCESSING,122(00),181-189.
MLA Sun, Yong,et al."Fischer-Trospch synthesis using iron-based catalyst in a microchannel reactor: Hybrid lump kinetic with ANNs/RSM".CHEMICAL ENGINEERING AND PROCESSING 122.00(2017):181-189.
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