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Recovery of Lithium, Nickel, and Cobalt from Spent Lithium-Ion Battery Powders by Selective Ammonia Leaching and an Adsorption Separation System
Wang, Hongyan1,2; Huang, Kai2; Zhang, Yang1; Chen, Xin1; Jin, Wei1; Zheng, Shili1; Zhang, Yi1; Li, Ping1
2017-12-01
发表期刊ACS SUSTAINABLE CHEMISTRY & ENGINEERING
ISSN2168-0485
卷号5期号:12页码:11489-11495
摘要

A novel hydrometallurgical route was developed to recover valuable metals from spent lithium-ion battery (LIB) powders. An ammonia media was utilized to selectively leach lithium, nickel, and cobalt from the pretreated spent LIB powders. Subsequently, an adsorption method was adopted to effectively separate lithium from Co2+ -Ni2+- -Li+ -NH4+-containing leaching solutions using manganese type lithium ion-sieves as adsorbents. The results showed that the direct recovery efficiencies of lithium, nickel, and cobalt from the spent LIB powders reached 76.19%, 96.23%, and 94.57%, respectively. Also, ammonia could be closed loop recycled, while Li2CO3, NiSO4, and CoSO4 could be obtained as products. This study provides a new pathway for recycling utilization of spent LIB powders.

关键词Spent Lithium-ion Ternary Batteries Recovery Ammonia Leaching Adsorption Separation Manganese Type Lithium Ion-sieves
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1021/acssuschemeng.7b02700
收录类别SCI
语种英语
关键词[WOS]Versatic 10 Acid ; Hydrometallurgical Process ; Cathode Materials ; Valuable Metals ; Tartaric Acid ; Manganese ; Extraction ; Removal ; Oxide ; Sieve
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Engineering
WOS类目Chemistry, Multidisciplinary ; Green & Sustainable Science & Technology ; Engineering, Chemical
项目资助者National Nature Science Foundation of China(51574212 ; U1403195)
WOS记录号WOS:000417341900040
引用统计
文献类型期刊论文
条目标识符http://ir.ipe.ac.cn/handle/122111/23499
专题研究所(批量导入)
通讯作者Li, Ping
作者单位1.Chinese Acad Sci, Key Lab Green Proc & Engn, Inst Proc Engn, Natl Engn Lab Hydrometallurg Cleaner Prod Technol, 1 North Second St, Beijing 100190, Peoples R China
2.Univ Sci & Technol Beijing, Sch Met & Ecol Engn, 30 Xueyuan Rd, Beijing 100083, Peoples R China
推荐引用方式
GB/T 7714
Wang, Hongyan,Huang, Kai,Zhang, Yang,et al. Recovery of Lithium, Nickel, and Cobalt from Spent Lithium-Ion Battery Powders by Selective Ammonia Leaching and an Adsorption Separation System[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2017,5(12):11489-11495.
APA Wang, Hongyan.,Huang, Kai.,Zhang, Yang.,Chen, Xin.,Jin, Wei.,...&Li, Ping.(2017).Recovery of Lithium, Nickel, and Cobalt from Spent Lithium-Ion Battery Powders by Selective Ammonia Leaching and an Adsorption Separation System.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,5(12),11489-11495.
MLA Wang, Hongyan,et al."Recovery of Lithium, Nickel, and Cobalt from Spent Lithium-Ion Battery Powders by Selective Ammonia Leaching and an Adsorption Separation System".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 5.12(2017):11489-11495.
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