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Recovery of Lithium, Nickel, and Cobalt from Spent Lithium-Ion Battery Powders by Selective Ammonia Leaching and an Adsorption Separation System
Wang, Hongyan1,2; Huang, Kai2; Zhang, Yang1; Chen, Xin1; Jin, Wei1; Zheng, Shili1; Zhang, Yi1; Li, Ping1
2017-12-01
Source PublicationACS SUSTAINABLE CHEMISTRY & ENGINEERING
ISSN2168-0485
Volume5Issue:12Pages:11489-11495
Abstract

A novel hydrometallurgical route was developed to recover valuable metals from spent lithium-ion battery (LIB) powders. An ammonia media was utilized to selectively leach lithium, nickel, and cobalt from the pretreated spent LIB powders. Subsequently, an adsorption method was adopted to effectively separate lithium from Co2+ -Ni2+- -Li+ -NH4+-containing leaching solutions using manganese type lithium ion-sieves as adsorbents. The results showed that the direct recovery efficiencies of lithium, nickel, and cobalt from the spent LIB powders reached 76.19%, 96.23%, and 94.57%, respectively. Also, ammonia could be closed loop recycled, while Li2CO3, NiSO4, and CoSO4 could be obtained as products. This study provides a new pathway for recycling utilization of spent LIB powders.

KeywordSpent Lithium-ion Ternary Batteries Recovery Ammonia Leaching Adsorption Separation Manganese Type Lithium Ion-sieves
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1021/acssuschemeng.7b02700
Indexed BySCI
Language英语
WOS KeywordVersatic 10 Acid ; Hydrometallurgical Process ; Cathode Materials ; Valuable Metals ; Tartaric Acid ; Manganese ; Extraction ; Removal ; Oxide ; Sieve
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Engineering
WOS SubjectChemistry, Multidisciplinary ; Green & Sustainable Science & Technology ; Engineering, Chemical
Funding OrganizationNational Nature Science Foundation of China(51574212 ; U1403195)
WOS IDWOS:000417341900040
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/23499
Collection研究所(批量导入)
Corresponding AuthorLi, Ping
Affiliation1.Chinese Acad Sci, Key Lab Green Proc & Engn, Inst Proc Engn, Natl Engn Lab Hydrometallurg Cleaner Prod Technol, 1 North Second St, Beijing 100190, Peoples R China
2.Univ Sci & Technol Beijing, Sch Met & Ecol Engn, 30 Xueyuan Rd, Beijing 100083, Peoples R China
Recommended Citation
GB/T 7714
Wang, Hongyan,Huang, Kai,Zhang, Yang,et al. Recovery of Lithium, Nickel, and Cobalt from Spent Lithium-Ion Battery Powders by Selective Ammonia Leaching and an Adsorption Separation System[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2017,5(12):11489-11495.
APA Wang, Hongyan.,Huang, Kai.,Zhang, Yang.,Chen, Xin.,Jin, Wei.,...&Li, Ping.(2017).Recovery of Lithium, Nickel, and Cobalt from Spent Lithium-Ion Battery Powders by Selective Ammonia Leaching and an Adsorption Separation System.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,5(12),11489-11495.
MLA Wang, Hongyan,et al."Recovery of Lithium, Nickel, and Cobalt from Spent Lithium-Ion Battery Powders by Selective Ammonia Leaching and an Adsorption Separation System".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 5.12(2017):11489-11495.
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