CAS OpenIR  > 湿法冶金清洁生产技术国家工程实验室
Performance Study of Stirred Tank Slurry Reactor and Fixed-Bed Reactor Using Bimetallic Co-Ni Mesoporous Silica Catalyst for Fischer-Tropsch Synthesis
Sun, Yong1; Yang, Gang2; Sun, Guangzhi1; Sun, Zhi3; Zhang, Lian4
2018
Source PublicationENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY
ISSN1944-7442
Volume37Issue:1Pages:553-561
AbstractThe Fischer-Tropsch synthesis (FTS) was studied using mesoporous silica-supported bimetallic Co-Ni catalyst in a fixed-bed reactor (FBR) and a slurry continuously stirred tank reactor (CSTR) under different temperatures (from 280 degrees C to 300 degrees C) with syngas ratio of 2 and a total pressure of 3.5 MPa. The activity of the catalyst was higher in FBR due to complete reduction. The CSTR was found to experience a less degree of catalyst deactivation, and its CO conversion was more sensitive in responding to the variation of temperatures because of its better temperature control. The intraparticle diffusion limitation was much improved in the CSTR system due to employment of smaller particle size of the catalyst. The selectivity of gasoline fraction (C-5-C-13) was higher in CSTR system than that in FBR at the same baseline condition. The appreciable increases of selectivity in CO2, methane, and longer-chain hydrocarbon were observed in FBR when the comparable CO conversion was set for comparison between FBR and CSTR. Reducing the particle size of the catalyst was more effective in increasing the selectivity of lighter (C-2-C-6) 1-olefin in CSTR system. The FBR produced higher selectivity of longer chain (C-7+) 1-olefin. (C) 2017 American Institute of Chemical Engineers
KeywordFischer-tropsch Synthesis Fixed-bed Reactor Slurry Continuous Stirred Tank Reactor
SubtypeArticle
WOS HeadingsScience & Technology ; Technology ; Life Sciences & Biomedicine
DOI10.1002/ep.12696
Indexed BySCI
Language英语
WOS KeywordHYDROCARBON SYNTHESIS ; REACTION PATHWAYS ; ACTIVATED CARBON ; MEMBRANE REACTOR ; HEAT-TRANSFER ; CHAIN-LENGTH ; IRON ; OPTIMIZATION ; METHANE ; WATER
WOS Research AreaScience & Technology - Other Topics ; Engineering ; Environmental Sciences & Ecology
WOS SubjectGREEN & SUSTAINABLE SCIENCE & TECHNOLOGY ; Engineering, Environmental ; Engineering, Chemical ; Engineering, Industrial ; Environmental Sciences
Funding OrganizationAnpeng high-tech energy and resource-company
WOS IDWOS:000419908200058
Citation statistics
Cited Times:2[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/24083
Collection湿法冶金清洁生产技术国家工程实验室
Affiliation1.Edith Cowan Univ, Sch Engn, Joondalup, WA 6027, Australia
2.Anpeng Energy Grp, Beijing 100190, Peoples R China
3.Chinese Acad Sci, Natl Engn Lab Hydromet Cleaner Prod Technol, Inst Proc Engn, Beijing 100190, Peoples R China
4.Monash Univ, Dept Chem Engn, Melbourne, Vic 3800, Australia
Recommended Citation
GB/T 7714
Sun, Yong,Yang, Gang,Sun, Guangzhi,et al. Performance Study of Stirred Tank Slurry Reactor and Fixed-Bed Reactor Using Bimetallic Co-Ni Mesoporous Silica Catalyst for Fischer-Tropsch Synthesis[J]. ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY,2018,37(1):553-561.
APA Sun, Yong,Yang, Gang,Sun, Guangzhi,Sun, Zhi,&Zhang, Lian.(2018).Performance Study of Stirred Tank Slurry Reactor and Fixed-Bed Reactor Using Bimetallic Co-Ni Mesoporous Silica Catalyst for Fischer-Tropsch Synthesis.ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY,37(1),553-561.
MLA Sun, Yong,et al."Performance Study of Stirred Tank Slurry Reactor and Fixed-Bed Reactor Using Bimetallic Co-Ni Mesoporous Silica Catalyst for Fischer-Tropsch Synthesis".ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY 37.1(2018):553-561.
Files in This Item:
There are no files associated with this item.
Related Services
Recommend this item
Bookmark
Usage statistics
Export to Endnote
Google Scholar
Similar articles in Google Scholar
[Sun, Yong]'s Articles
[Yang, Gang]'s Articles
[Sun, Guangzhi]'s Articles
Baidu academic
Similar articles in Baidu academic
[Sun, Yong]'s Articles
[Yang, Gang]'s Articles
[Sun, Guangzhi]'s Articles
Bing Scholar
Similar articles in Bing Scholar
[Sun, Yong]'s Articles
[Yang, Gang]'s Articles
[Sun, Guangzhi]'s Articles
Terms of Use
No data!
Social Bookmark/Share
All comments (0)
No comment.
 

Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.