CAS OpenIR
Catalytic oxidation of ethyl acetate over LaBO3 (B = Co, Mn, Ni, Fe) perovskites supported silver catalysts
Qin, Yu1; Shen, Fangxia1; Zhu, Tianle1; Hong, Wei1; Liu, Xiaolong2
2018
Source PublicationRSC ADVANCES
ISSN2046-2069
Volume8Issue:58Pages:33425-33431
Abstract

A series of silver catalysts supported on lanthanum based perovskites LaBO3 (B = Co, Mn, Ni, Fe) were synthesized and evaluated in the catalytic oxidation of ethyl acetate. XRD, BET, TEM/HRTEM, HAADF-STEM, XPS and H-2-TPR were conducted, and the results indicate that redox activity of the catalysts is of great importance to the oxidation reaction. Activity tests demonstrated that Ag/LaCoO3 was more active than the other samples in ethyl acetate oxidation. Moreover, the CO2 selectivity, COx yields and byproduct distributions for all catalysts were studied, and Ag/LaCoO3 showed the best catalytic performance. Besides, Ag/LaCoO3 also showed excellent catalytic activity for other OVOCs.

DOI10.1039/c8ra06933f
Language英语
WOS KeywordVolatile Organic-compounds ; Lacoo3 Perovskite ; Surface-properties ; Toluene Oxidation ; Metal-catalysts ; Oxides ; Performance ; Combustion ; Generation ; Lanthanum
Funding ProjectNational Key R&D Program of China[2016YFC0207103] ; Natural Science Foundation of China[21607154]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationNational Key R&D Program of China ; Natural Science Foundation of China
WOS IDWOS:000448422800050
PublisherROYAL SOC CHEMISTRY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/26408
Collection中国科学院过程工程研究所
Corresponding AuthorLiu, Xiaolong
Affiliation1.Beihang Univ, Sch Space & Environm, Beijing 100191, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, Natl Engn Lab Hydromet Cleaner Prod Technol, Beijing Engn Res Ctr Proc Pollut Control, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Qin, Yu,Shen, Fangxia,Zhu, Tianle,et al. Catalytic oxidation of ethyl acetate over LaBO3 (B = Co, Mn, Ni, Fe) perovskites supported silver catalysts[J]. RSC ADVANCES,2018,8(58):33425-33431.
APA Qin, Yu,Shen, Fangxia,Zhu, Tianle,Hong, Wei,&Liu, Xiaolong.(2018).Catalytic oxidation of ethyl acetate over LaBO3 (B = Co, Mn, Ni, Fe) perovskites supported silver catalysts.RSC ADVANCES,8(58),33425-33431.
MLA Qin, Yu,et al."Catalytic oxidation of ethyl acetate over LaBO3 (B = Co, Mn, Ni, Fe) perovskites supported silver catalysts".RSC ADVANCES 8.58(2018):33425-33431.
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