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Immobilizing Ultrafine PtNi Nanoparticles within Graphitic Carbon Nanosheets toward High-Performance Hydrogenation Reaction
Xu, Linlin1; Zhang, Jingfei3; Xu, Lin3; Yang, Jun1,2
2018-12-01
Source PublicationACS OMEGA
ISSN2470-1343
Volume3Issue:12Pages:16436-16442
Abstract

Immobilization of Pt-based nanoparticles on carbon support is of great significance in catalysis for their superior activity and enhanced durability. Herein, we report for the first time a feasible NaCl template-engaged approach to firmly immobilize PtNi nanoparticles into two-dimensional (2D) graphitic carbon nanosheets (denoted as PtNi@GCNs hereafter). The elaborate employment of the NaCl template regulates the formation of 2D graphitic carbon nanosheets, which tightly immobilize the in situ-generated PtNi nanoparticles. The smart integration of catalytically active PtNi nanoparticles with carbon nanosheets endows the as-prepared PtNi@GCNs with superior catalytic activity and outstanding stability toward the hydrogenation of 4-nitrophenol, making them a promising catalyst for environmental remediation. We believe that the present work can inspire the future design of carbon nanosheet-based nanohybrids with unique functionalities for diverse applications.

DOI10.1021/acsomega.8b02746
Language英语
WOS KeywordFormaldehyde Oxidation ; Facile Synthesis ; Selective Reduction ; Catalytic-activity ; Pd Nanoparticles ; Size ; Methanol ; Tio2 ; Au ; Electrocatalysts
Funding ProjectNational Natural Science Foundation of China[21503111] ; National Natural Science Foundation of China[21573240] ; Natural Science Foundation of Jiangsu Higher Education Institutions of China[16KJB150020] ; Natural Science Foundation of Jiangsu Province[BK20171473] ; Center for Mesoscience, Institute of Process Engineering, Chinese Academy of Sciences[COM2015A001] ; Center for Mesoscience, Institute of Process Engineering, Chinese Academy of Sciences[MPCS-2017-A-02] ; 2017 Jurong SME Technology Innovation Project[CX2017006]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationNational Natural Science Foundation of China ; Natural Science Foundation of Jiangsu Higher Education Institutions of China ; Natural Science Foundation of Jiangsu Province ; Center for Mesoscience, Institute of Process Engineering, Chinese Academy of Sciences ; 2017 Jurong SME Technology Innovation Project
WOS IDWOS:000454244600006
PublisherAMER CHEMICAL SOC
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/27648
Collection中国科学院过程工程研究所
Corresponding AuthorXu, Lin; Yang, Jun
Affiliation1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, Ctr Mesosci, Beijing 100190, Peoples R China
3.Nanjing Normal Univ, Sch Chem & Mat Sci, Jiangsu Collaborate Innovat Ctr Biomed Funct Mat, Jiangsu Key Lab New Power Batteries, Nanjing 210023, Jiangsu, Peoples R China
Recommended Citation
GB/T 7714
Xu, Linlin,Zhang, Jingfei,Xu, Lin,et al. Immobilizing Ultrafine PtNi Nanoparticles within Graphitic Carbon Nanosheets toward High-Performance Hydrogenation Reaction[J]. ACS OMEGA,2018,3(12):16436-16442.
APA Xu, Linlin,Zhang, Jingfei,Xu, Lin,&Yang, Jun.(2018).Immobilizing Ultrafine PtNi Nanoparticles within Graphitic Carbon Nanosheets toward High-Performance Hydrogenation Reaction.ACS OMEGA,3(12),16436-16442.
MLA Xu, Linlin,et al."Immobilizing Ultrafine PtNi Nanoparticles within Graphitic Carbon Nanosheets toward High-Performance Hydrogenation Reaction".ACS OMEGA 3.12(2018):16436-16442.
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