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Study on the Catalytic Properties of Ru/TiO2 Catalysts for the Catalytic Oxidation of (Chloro)-Aromatics
Wang, Jian1; Zhao, Hainan1,3; Liu, Xiaolong1; Xu, Wenqing1,2; Guo, Yangyang1; Song, Jianfei3; Zhu, Tingyu1,2
2019-07-01
Source PublicationCATALYSIS LETTERS
ISSN1011-372X
Volume149Issue:7Pages:2004-2014
AbstractIn this work, we presented a detailed evaluation of Ru/TiO2 (P25) catalysts for the catalytic oxidation of (chloro)-aromatics. The model catalysts were synthesized through wet impregnation. Catalytic evaluations, as well as ICP, BET, XRD and TEM analyses, were conducted. The results indicated that RuO2 tended to be distributed on the rutile phase of TiO2, leading to an inhomogeneous distribution. These Ru/TiO2 catalysts were very active, especially for chlorobenzene oxidation. The conversions of benzene and chlorobenzene were both suppressed by the introduction of additional water. But the amount of polychlorinated benzenes as by-products was also reduced. However, the activity of the catalyst significantly decreased with an increase in calcination temperature, suggesting that the thermal stability of the catalyst still needed to be improved. [GRAPHICS] .
KeywordRuthenium Ru TiO2 Catalytic oxidation Benzene Chlorobenzene
DOI10.1007/s10562-019-02802-x
Language英语
WOS KeywordRUTHENIUM CATALYSTS ; RU/CEO2 CATALYSTS ; AMMONIA-SYNTHESIS ; LOW-TEMPERATURE ; COMBUSTION ; CHLOROBENZENE ; VOCS ; CO ; EMISSION ; KINETICS
Funding ProjectNational Natural Science Foundation of China[51708540] ; Key Research Program of the Chinese Academy of Sciences[ZDRW-ZS-2017-6-2]
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
Funding OrganizationNational Natural Science Foundation of China ; Key Research Program of the Chinese Academy of Sciences
WOS IDWOS:000468172400026
PublisherSPRINGER
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/28149
Collection中国科学院过程工程研究所
Corresponding AuthorWang, Jian; Zhu, Tingyu
Affiliation1.Chinese Acad Sci, Beijing Res Ctr Proc Pollut Control, Inst Proc Engn, Natl Engn Lab Hydromet Cleaner Prod Technol, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China
3.China Univ Petr, Coll Mech & Transportat Engn, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China
Recommended Citation
GB/T 7714
Wang, Jian,Zhao, Hainan,Liu, Xiaolong,et al. Study on the Catalytic Properties of Ru/TiO2 Catalysts for the Catalytic Oxidation of (Chloro)-Aromatics[J]. CATALYSIS LETTERS,2019,149(7):2004-2014.
APA Wang, Jian.,Zhao, Hainan.,Liu, Xiaolong.,Xu, Wenqing.,Guo, Yangyang.,...&Zhu, Tingyu.(2019).Study on the Catalytic Properties of Ru/TiO2 Catalysts for the Catalytic Oxidation of (Chloro)-Aromatics.CATALYSIS LETTERS,149(7),2004-2014.
MLA Wang, Jian,et al."Study on the Catalytic Properties of Ru/TiO2 Catalysts for the Catalytic Oxidation of (Chloro)-Aromatics".CATALYSIS LETTERS 149.7(2019):2004-2014.
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