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Synthesis and Applications of Graphdiyne-Based Metal-Free Catalysts
Zuo, Zicheng1; Wang, Dan2; Zhang, Jin3; Lu, Fushen4,5; Li, Yuliang1,6
2019-03-27
Source PublicationADVANCED MATERIALS
ISSN0935-9648
Volume31Issue:13Pages:13
Abstract

The development of carbon materials offers the hope for obtaining inexpensive and high-performance alternatives to substitute noble-metal catalysts for their sustainable application. Graphdiyne, the rising-star carbon allotrope, is a big family with many members, and first realized the coexistence of sp- and sp(2) hybridized carbon atoms in a 2D planar structure. Different from the prevailing carbon materials, its nonuniform distribution in the electronic structure and wide tunability in bandgap show many possibilities and special inspirations to construct new-concept metal-free catalysts, and provide many opportunities for achieving a catalytic activity comparable with that of noble-metal catalysts. Herein, the recent progress in synthetic methodologies, theoretical predictions, and experimental investigations of graphdiyne for metal-free catalysts is systematically summarized. Some new perspectives of the opportunities and challenges in developing high-performance graphdiyne-based metal-free catalysts are demonstrated.

KeywordGraphdiyne Metal-free Catalysts Oxygen Reduction Reaction Photocatalysts Water Splitting
DOI10.1002/adma.201803762
Language英语
WOS KeywordNitrogen-doped Graphdiyne ; Oxygen Reduction Reaction ; Hydrogen-storage ; Low-temperature ; Electrocatalytic Activities ; Electronic-properties ; Carbon ; Graphene ; Graphyne ; Boron
Funding ProjectNational Nature Science Foundation of China[21790050] ; National Nature Science Foundation of China[21790051] ; National Key Research and Development Project of China[2016YFA0200104] ; Key Program of the Chinese Academy of Sciences[QYZDY-SSW-SLH015]
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS SubjectChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
Funding OrganizationNational Nature Science Foundation of China ; National Key Research and Development Project of China ; Key Program of the Chinese Academy of Sciences
WOS IDWOS:000463970200004
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/28273
Collection中国科学院过程工程研究所
Corresponding AuthorLi, Yuliang
Affiliation1.Chinese Acad Sci, Beijing Natl Lab Mol Sci, CAS Res Educ Ctr Excellence Mol Sci, Inst Chem,CAS Key Lab Organ Solids, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China
3.Peking Univ, Coll Chem & Mol Engn, Beijing 100871, Peoples R China
4.Shantou Univ, Dept Chem, Shantou 515063, Guangdong, Peoples R China
5.Shantou Univ, Guangdong Key Lab Preparat & Applicat Ordered Str, Shantou 515063, Guangdong, Peoples R China
6.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Zuo, Zicheng,Wang, Dan,Zhang, Jin,et al. Synthesis and Applications of Graphdiyne-Based Metal-Free Catalysts[J]. ADVANCED MATERIALS,2019,31(13):13.
APA Zuo, Zicheng,Wang, Dan,Zhang, Jin,Lu, Fushen,&Li, Yuliang.(2019).Synthesis and Applications of Graphdiyne-Based Metal-Free Catalysts.ADVANCED MATERIALS,31(13),13.
MLA Zuo, Zicheng,et al."Synthesis and Applications of Graphdiyne-Based Metal-Free Catalysts".ADVANCED MATERIALS 31.13(2019):13.
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