CAS OpenIR
Metal Ionic Liquids Produce Metal-Dispersed Carbon-Nitrogen Networks for Efficient CO2 Electroreduction
Cheng, Xiuyan1,2; Tan, Dongxing1,2; Zeng, Shaojuan3; Zhang, Xiangping3; Tan, Xiuniang1,2; Shi, Jinbiao1,2; Zhang, Bingxing1,2; Zheng, Lirong4; Zhang, Fanyu1,2; Feng, Jiaqi3; Liu, Lifei1,2; Wan, Qiang1,2; Chen, Gang1,2; Han, Buxing1,2,5; Zhang, Jing4; An, Pengfei4; Zhang, Jianling1,2,5
2019-07-18
Source PublicationCHEMCATCHEM
ISSN1867-3880
Volume11Issue:14Pages:3166-3170
AbstractTo develop novel strategies for fabricating metal carbon-based materials with desirable compositions and structures for catalysis is of great importance. Here we propose for the first time the utilization of metal ionic liquid as a precursor for the synthesis of metal carbon-based materials through a one-step pyrolysis route. The method produces the metal dispersed cross-linked carbon framework with a highly mesoporous structure. Such a Ni/C-N catalyst exhibits outstanding electrocatalytic activity for CO2 reduction reaction, i. e., an excellent CO faradaic efficiency of approximately 94 % at an potential of -0.75 V (versus the reversible hydrogen electrode). The method proposed in this work is simple, convenient, low-cost, adjustable and versatile for the synthesis of different kinds of M/C-N materials because the structures and properties of metal ionic liquids can be easily designed and tuned by changing the anions and cations.
Keywordmetal ionic liquid CO2 reduction coordination electrocatalyst
DOI10.1002/cctc.201900615
Language英语
WOS KeywordREDUCTION ; CATALYSIS ; SITES
Funding ProjectNational Natural Science Foundation of China[21525316] ; National Natural Science Foundation of China[21673254] ; Ministry of Science and Technology of China[2017YFA0403003] ; Chinese Academy of Sciences[QYZDY-SSW-SLH013] ; Beijing Municipal Science & Technology Commission[Z181100004218004]
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
Funding OrganizationNational Natural Science Foundation of China ; Ministry of Science and Technology of China ; Chinese Academy of Sciences ; Beijing Municipal Science & Technology Commission
WOS IDWOS:000477986300004
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/30320
Collection中国科学院过程工程研究所
Corresponding AuthorZhang, Jianling
Affiliation1.Chinese Acad Sci, Beijing Natl Lab Mol Sci, CAS Key Lab Colloid Interface & Chem Thermodynam, CAS Res Educ Ctr Excellence Mol Sci,Inst Chem, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Sch Chem Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China
4.Chinese Acad Sci, BSRF, Inst High Energy Phys, Beijing 100049, Peoples R China
5.Huairou Natl Comprehens Sci Ctr, Phys Sci Lab, Beijing 101400, Peoples R China
Recommended Citation
GB/T 7714
Cheng, Xiuyan,Tan, Dongxing,Zeng, Shaojuan,et al. Metal Ionic Liquids Produce Metal-Dispersed Carbon-Nitrogen Networks for Efficient CO2 Electroreduction[J]. CHEMCATCHEM,2019,11(14):3166-3170.
APA Cheng, Xiuyan.,Tan, Dongxing.,Zeng, Shaojuan.,Zhang, Xiangping.,Tan, Xiuniang.,...&Zhang, Jianling.(2019).Metal Ionic Liquids Produce Metal-Dispersed Carbon-Nitrogen Networks for Efficient CO2 Electroreduction.CHEMCATCHEM,11(14),3166-3170.
MLA Cheng, Xiuyan,et al."Metal Ionic Liquids Produce Metal-Dispersed Carbon-Nitrogen Networks for Efficient CO2 Electroreduction".CHEMCATCHEM 11.14(2019):3166-3170.
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