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A Rutile TiO2 Electron Transport Layer for the Enhancement of Charge Collection for Efficient Perovskite Solar Cells | |
Wang, Yongling1,2; Wan, Jiawei1; Ding, Jie2,3; Hu, Jin-Song2,3; Wang, Dan1,2 | |
2019-07-08 | |
Source Publication | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
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ISSN | 1433-7851 |
Volume | 58Issue:28Pages:9414-9418 |
Abstract | Interfacial charge collection efficiency has demonstrated significant effects on the power conversion efficiency (PCE) of perovskite solar cells (PSCs). Herein, crystalline phase-dependent charge collection is investigated by using rutile and anatase TiO2 electron transport layer (ETL) to fabricate PSCs. The results show that rutile TiO2 ETL enhances the extraction and transportation of electrons to FTO and reduces the recombination, thanks to its better conductivity and improved interface with the CH3NH3PbI3 (MAPbI(3)) layer. Moreover, this may be also attributed to the fact that rutile TiO2 has better match with perovskite grains, and less trap density. As a result, comparing with anatase TiO2 ETL, MAPbI(3) PSCs with rutile TiO2 ETL delivers significantly enhanced performance with a champion PCE of 20.9% and a large open circuit voltage (V-OC) of 1.17V. |
Keyword | Electron Lifetime Interfaces Open Circuit Voltage Perovskite Solar Cells Rutile Tio2 |
DOI | 10.1002/anie.201902984 |
Language | 英语 |
WOS Keyword | Hollow Microspheres ; Performance ; Films |
Funding Project | National Natural Science Foundation of China[21590795] ; National Natural Science Foundation of China[21820102002] ; National Natural Science Foundation of China[51802306] ; Scientific Instrument Developing Project of the Chinese Academy of Sciences[YZ201623] ; Queensland-Chinese Academy of Sciences Collaborative Science Fund[122111KYSB20170001] ; Chinese Academy of Sciences (CAS) Interdisciplinary Innovation Team |
WOS Research Area | Chemistry |
WOS Subject | Chemistry, Multidisciplinary |
Funding Organization | National Natural Science Foundation of China ; Scientific Instrument Developing Project of the Chinese Academy of Sciences ; Queensland-Chinese Academy of Sciences Collaborative Science Fund ; Chinese Academy of Sciences (CAS) Interdisciplinary Innovation Team |
WOS ID | WOS:000476610900015 |
Publisher | WILEY-V C H VERLAG GMBH |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.ipe.ac.cn/handle/122111/30408 |
Collection | 中国科学院过程工程研究所 |
Corresponding Author | Hu, Jin-Song; Wang, Dan |
Affiliation | 1.Chinese Acad Sci, State Key Lab Biochem Engn, Inst Proc Engn, 1 North 2nd St, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China 3.Chinese Acad Sci, BNLMS, CAS Key Lab Mol Nanostruct & Nanotechnol, Inst Chem, Zhongguancun North First St 2, Beijing 100190, Peoples R China |
Recommended Citation GB/T 7714 | Wang, Yongling,Wan, Jiawei,Ding, Jie,et al. A Rutile TiO2 Electron Transport Layer for the Enhancement of Charge Collection for Efficient Perovskite Solar Cells[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2019,58(28):9414-9418. |
APA | Wang, Yongling,Wan, Jiawei,Ding, Jie,Hu, Jin-Song,&Wang, Dan.(2019).A Rutile TiO2 Electron Transport Layer for the Enhancement of Charge Collection for Efficient Perovskite Solar Cells.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,58(28),9414-9418. |
MLA | Wang, Yongling,et al."A Rutile TiO2 Electron Transport Layer for the Enhancement of Charge Collection for Efficient Perovskite Solar Cells".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 58.28(2019):9414-9418. |
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A Rutile TiO2 Electr(2936KB) | 期刊论文 | 出版稿 | 限制开放 | CC BY-NC-SA | Application Full Text |
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