CAS OpenIR  > 湿法冶金清洁生产技术国家工程实验室
Carbon capture with ionic liquids: overview and progress
Zhang, Xiangping3; Zhang, Xiaochun3; Dong, Haifeng3; Zhao, Zhijun3,4; Zhang, Suojiang3; Huang, Ying3,4; Zhang, XP
2012-05-01
Source PublicationENERGY & ENVIRONMENTAL SCIENCE
ISSN1754-5692
Volume5Issue:5Pages:6668-6681
AbstractAs an emerging carbon dioxide (CO2) capture technology, separating CO2 from industrial gases with ionic liquids is increasingly attracting remarkable interests. In this paper, the research progress on CO2 capture with ionic liquids is reviewed with particular attention on the viewpoint of potential industrial applications. We investigate and compare the CO2 capture capacities of pure ionic liquids, including conventional and task-specific ionic liquids, and ionic liquid-based mixtures. The mechanisms of chemisorption and physisorption are explained with experimental characteristics and molecular simulation, which show more and more important roles for screening suitable ionic liquids from tremendous candidates. Considering the scaling up of novel units for ionic liquid-based fluids, the studies on the transport properties and hydrodynamics of ionic liquid fluids are presented. The process design and assessment of ionic liquid processes are discussed, including the research progress on thermodynamic properties and prediction models. Besides giving an overview of research for each issue above, we also provide discussions for future work to try to identify the gap between the current work and the demand by real industrial applications. Finally, we present some perspectives of ionic liquid-based novel technologies, and the challenges which will be faced while developing industrially available technologies.
KeywordPressure Phase-behavior Life-cycle Assessment Co2 Capture Dioxide Capture Molecular-dynamics Elevated Pressures 1-ethyl-3-methylimidazolium Tetrafluoroborate Aqueous-solutions Power-plant Cosmo-rs
SubtypeReview
WOS HeadingsScience & Technology ; Physical Sciences ; Technology ; Life Sciences & Biomedicine
DOI10.1039/c2ee21152a
Indexed BySCI
Language英语
WOS KeywordPRESSURE PHASE-BEHAVIOR ; LIFE-CYCLE ASSESSMENT ; CO2 CAPTURE ; DIOXIDE CAPTURE ; MOLECULAR-DYNAMICS ; ELEVATED PRESSURES ; 1-ETHYL-3-METHYLIMIDAZOLIUM TETRAFLUOROBORATE ; AQUEOUS-SOLUTIONS ; POWER-PLANT ; COSMO-RS
WOS Research AreaChemistry ; Energy & Fuels ; Engineering ; Environmental Sciences & Ecology
WOS SubjectChemistry, Multidisciplinary ; Energy & Fuels ; Engineering, Chemical ; Environmental Sciences
WOS IDWOS:000303251500005
Citation statistics
Document Type期刊论文
Version出版稿
Identifierhttp://ir.ipe.ac.cn/handle/122111/3829
Collection湿法冶金清洁生产技术国家工程实验室
Corresponding AuthorZhang, XP
Affiliation1.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Coll Chem & Chem Engn, Grad Univ, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing 100190, Peoples R China
4.Chinese Acad Sci, Coll Chem & Chem Engn, Grad Univ, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Xiangping,Zhang, Xiaochun,Dong, Haifeng,et al. Carbon capture with ionic liquids: overview and progress[J]. ENERGY & ENVIRONMENTAL SCIENCE,2012,5(5):6668-6681.
APA Zhang, Xiangping.,Zhang, Xiaochun.,Dong, Haifeng.,Zhao, Zhijun.,Zhang, Suojiang.,...&Zhang, XP.(2012).Carbon capture with ionic liquids: overview and progress.ENERGY & ENVIRONMENTAL SCIENCE,5(5),6668-6681.
MLA Zhang, Xiangping,et al."Carbon capture with ionic liquids: overview and progress".ENERGY & ENVIRONMENTAL SCIENCE 5.5(2012):6668-6681.
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