Carbon capture with ionic liquids: overview and progress
Zhang, Xiangping3; Zhang, Xiaochun3; Dong, Haifeng3; Zhao, Zhijun3,4; Zhang, Suojiang3; Huang, Ying3,4; Zhang, XP
2012-05-01
发表期刊ENERGY & ENVIRONMENTAL SCIENCE
ISSN1754-5692
卷号5期号:5页码:6668-6681
摘要As an emerging carbon dioxide (CO2) capture technology, separating CO2 from industrial gases with ionic liquids is increasingly attracting remarkable interests. In this paper, the research progress on CO2 capture with ionic liquids is reviewed with particular attention on the viewpoint of potential industrial applications. We investigate and compare the CO2 capture capacities of pure ionic liquids, including conventional and task-specific ionic liquids, and ionic liquid-based mixtures. The mechanisms of chemisorption and physisorption are explained with experimental characteristics and molecular simulation, which show more and more important roles for screening suitable ionic liquids from tremendous candidates. Considering the scaling up of novel units for ionic liquid-based fluids, the studies on the transport properties and hydrodynamics of ionic liquid fluids are presented. The process design and assessment of ionic liquid processes are discussed, including the research progress on thermodynamic properties and prediction models. Besides giving an overview of research for each issue above, we also provide discussions for future work to try to identify the gap between the current work and the demand by real industrial applications. Finally, we present some perspectives of ionic liquid-based novel technologies, and the challenges which will be faced while developing industrially available technologies.
关键词Pressure Phase-behavior Life-cycle Assessment Co2 Capture Dioxide Capture Molecular-dynamics Elevated Pressures 1-ethyl-3-methylimidazolium Tetrafluoroborate Aqueous-solutions Power-plant Cosmo-rs
文章类型Review
WOS标题词Science & Technology ; Physical Sciences ; Technology ; Life Sciences & Biomedicine
DOI10.1039/c2ee21152a
收录类别SCI
语种英语
关键词[WOS]PRESSURE PHASE-BEHAVIOR ; LIFE-CYCLE ASSESSMENT ; CO2 CAPTURE ; DIOXIDE CAPTURE ; MOLECULAR-DYNAMICS ; ELEVATED PRESSURES ; 1-ETHYL-3-METHYLIMIDAZOLIUM TETRAFLUOROBORATE ; AQUEOUS-SOLUTIONS ; POWER-PLANT ; COSMO-RS
WOS研究方向Chemistry ; Energy & Fuels ; Engineering ; Environmental Sciences & Ecology
WOS类目Chemistry, Multidisciplinary ; Energy & Fuels ; Engineering, Chemical ; Environmental Sciences
WOS记录号WOS:000303251500005
引用统计
被引频次:373[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
版本出版稿
条目标识符http://ir.ipe.ac.cn/handle/122111/3829
专题湿法冶金清洁生产技术国家工程实验室
通讯作者Zhang, XP
作者单位1.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Coll Chem & Chem Engn, Grad Univ, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing 100190, Peoples R China
4.Chinese Acad Sci, Coll Chem & Chem Engn, Grad Univ, Beijing 100049, Peoples R China
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GB/T 7714
Zhang, Xiangping,Zhang, Xiaochun,Dong, Haifeng,et al. Carbon capture with ionic liquids: overview and progress[J]. ENERGY & ENVIRONMENTAL SCIENCE,2012,5(5):6668-6681.
APA Zhang, Xiangping.,Zhang, Xiaochun.,Dong, Haifeng.,Zhao, Zhijun.,Zhang, Suojiang.,...&Zhang, XP.(2012).Carbon capture with ionic liquids: overview and progress.ENERGY & ENVIRONMENTAL SCIENCE,5(5),6668-6681.
MLA Zhang, Xiangping,et al."Carbon capture with ionic liquids: overview and progress".ENERGY & ENVIRONMENTAL SCIENCE 5.5(2012):6668-6681.
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