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Formation and toxicity of polycyclic aromatic hydrocarbons during CaO assisted hydrothermal carbonization of swine manure | |
Lang, Qianqian1,2; Zhang, Bo3; Li, Yi4; Liu, Zhengang1,2; Jiao, Wentao1,2 | |
2019-12-01 | |
Source Publication | WASTE MANAGEMENT
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ISSN | 0956-053X |
Volume | 100Pages:84-90 |
Abstract | The effects of temperature and Ca0 introduction on polycyclic aromatic hydrocarbons (PAHs) contents, distribution patterns and toxicity of the products from hydrothermal carbonization (HTC) of swine manure (SM) were investigated in this study for the first time. The results indicated that increasing temperature decreased total PAHs content of the hydrochar, while the PAHs toxicity firstly decreased and then increased during HTC of SM. For the aqueous product, the total PAHs content and toxicity gradually decreased with increasing temperature. CaO introduction during HTC of SM significantly suppressed the PAHs formation and promoted the transformation from higher molecular weight PAHs into lower molecular weight PAHs in HTC products, resulting in the remarkably decreased content and toxicity of PAHs. The lowest total PAHs content (1428.57 mu g/kg) and TEQ value (21.33 mu g/kg) of the hydrochar were obtained by 15% CaO introduction at 200 degrees C and 180 degrees C, respectively, and compared to SM, they were decreased by 73.73% and 79.51%, respectively. Moreover, 3-ring PAHs were the predominant PAHs in HTC products regardless of CaO introduction. The present study demonstrated that CaO assisted HTC at temperature lower than 220 degrees C was effective to reduce the total content and toxicity of PAHs in SM, and the prepared hydrochar was a promising soil amendment in view of the elimination of PAHs toxicity. (C) 2019 Elsevier Ltd. All rights reserved. |
Keyword | Hydrothermal carbonization Swine manure CaO introduction Polycyclic aromatic hydrocarbons Soil amendment |
DOI | 10.1016/j.wasman.2019.09.010 |
Language | 英语 |
WOS Keyword | SEWAGE-SLUDGE ; HYDROCHAR ; PYROLYSIS ; PAHS ; SOIL ; BIOMASS ; WATER ; IDENTIFICATION ; GASIFICATION ; TEMPERATURE |
Funding Project | "100 Talents" Program of the Chinese Academy of Sciences[Y5N41I1C01] ; Science and Technology Department of Sichuan Province[2018YZ0016] |
WOS Research Area | Engineering ; Environmental Sciences & Ecology |
WOS Subject | Engineering, Environmental ; Environmental Sciences |
Funding Organization | "100 Talents" Program of the Chinese Academy of Sciences ; Science and Technology Department of Sichuan Province |
WOS ID | WOS:000494887900010 |
Publisher | PERGAMON-ELSEVIER SCIENCE LTD |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.ipe.ac.cn/handle/122111/38949 |
Collection | 中国科学院过程工程研究所 |
Corresponding Author | Liu, Zhengang; Jiao, Wentao |
Affiliation | 1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Shandong Prov Environm Technol Serv Ctr, Jinan 250102, Shandong, Peoples R China 4.Chinese Acad Sci, IPE, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China |
Recommended Citation GB/T 7714 | Lang, Qianqian,Zhang, Bo,Li, Yi,et al. Formation and toxicity of polycyclic aromatic hydrocarbons during CaO assisted hydrothermal carbonization of swine manure[J]. WASTE MANAGEMENT,2019,100:84-90. |
APA | Lang, Qianqian,Zhang, Bo,Li, Yi,Liu, Zhengang,&Jiao, Wentao.(2019).Formation and toxicity of polycyclic aromatic hydrocarbons during CaO assisted hydrothermal carbonization of swine manure.WASTE MANAGEMENT,100,84-90. |
MLA | Lang, Qianqian,et al."Formation and toxicity of polycyclic aromatic hydrocarbons during CaO assisted hydrothermal carbonization of swine manure".WASTE MANAGEMENT 100(2019):84-90. |
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