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Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible-Light CO2 Reduction with a SnS2/SnO2 Junction
You, Feifei1,2; Wan, Jiawei1; Qi, Jian1,2; Mao, Dan1,2; Yang, Nailiang1,2; Zhang, Qinghua3; Gu, Lin3; Wang, Dan1,2
2020-01-07
Source PublicationANGEWANDTE CHEMIE-INTERNATIONAL EDITION
ISSN1433-7851
Volume59Issue:2Pages:721-724
AbstractPrecise control of the micro-/nanostructures of nanomaterials, such as hollow multi-shelled structures (HoMSs), has shown its great advantages in various applications. Now, the crystal structure of building blocks of HoMSs are controlled by introducing the lattice distortion in HoMSs, for the first time. The lattice distortion located at the nanoscale interface of SnS2/SnO2 can provide additional active sites, which not only provide the catalytic activity under visible light but also improve the separation of photoexcited electron-hole pairs. Combined with the efficient light utilization, the natural advantage of HoMSs, a record catalytic activity was achieved in solid-gas system for CO2 reduction, with an excellent stability and 100% CO selectivity without using any sensitizers or noble metals.
KeywordCO2 photoreduction hollow structures lattice distortion multi-shells tin
DOI10.1002/ange.201912069
Language英语
WOS KeywordMICROSPHERES ; PHOTOCATALYSTS ; PERFORMANCE
Funding ProjectNational Natural Science Foundation of China[21590795] ; National Natural Science Foundation of China[21821005] ; National Natural Science Foundation of China[51772296] ; National Natural Science Foundation of China[51772294] ; National Natural Science Foundation of China[51702321] ; National Natural Science Foundation of China[51972306] ; National Natural Science Foundation of China[51802306] ; National Key R&D Program of China[2016YFB0600903] ; Youth Innovation Promotion Association of CAS[2017070]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationNational Natural Science Foundation of China ; National Key R&D Program of China ; Youth Innovation Promotion Association of CAS
WOS IDWOS:000505279500029
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/39205
Collection中国科学院过程工程研究所
Corresponding AuthorWang, Dan
Affiliation1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 10049, Peoples R China
3.Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
You, Feifei,Wan, Jiawei,Qi, Jian,et al. Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible-Light CO2 Reduction with a SnS2/SnO2 Junction[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2020,59(2):721-724.
APA You, Feifei.,Wan, Jiawei.,Qi, Jian.,Mao, Dan.,Yang, Nailiang.,...&Wang, Dan.(2020).Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible-Light CO2 Reduction with a SnS2/SnO2 Junction.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,59(2),721-724.
MLA You, Feifei,et al."Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible-Light CO2 Reduction with a SnS2/SnO2 Junction".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 59.2(2020):721-724.
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