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Polyoxometalates on Functional Substrates: Concepts, Synergies, and Future Perspectives
Cherevan, Alexey S.1; Nandan, Sreejith P.1; Roger, Isolda2; Liu, Rongji2,3; Streb, Carsten2,4; Eder, Dominik1
2020-04-01
Source PublicationADVANCED SCIENCE
Volume7Issue:8Pages:23
AbstractPolyoxometalates (POMs) are molecular metal oxide clusters that feature a broad range of structures and functionalities, making them one of the most versatile classes of inorganic molecular materials. They have attracted widespread attention in homogeneous catalysis. Due to the challenges associated with their aggregation, precipitation, and degradation under operational conditions and to extend their scope of applications, various strategies of depositing POMs on heterogeneous substrates have been developed. Recent ground-breaking developments in the materials chemistry of supported POM composites are summarized and links between molecular-level understanding of POM-support interactions and macroscopic effects including new or optimized reactivities, improved stability, and novel function are established. Current limitations and future challenges in studying these complex composite materials are highlighted, and cutting-edge experimental and theoretical methods that will lead to an improved understanding of synergisms between POM and support material from the molecular through to the nano- and micrometer level are discussed. Future development in this fast-moving field is explored and emerging fields of research in POM heterogenization are identified.
Keywordcharge transfer composites heterogenization molecular metal oxides substrates
DOI10.1002/advs.201903511
Language英语
WOS KeywordMETAL-ORGANIC FRAMEWORKS ; GRAPHITIC CARBON NITRIDE ; WATER OXIDATION CATALYST ; HIGHLY EFFICIENT ; KEGGIN-TYPE ; TIO2 NANOPARTICLES ; ELECTRON-TRANSFER ; PHOTOCATALYTIC DEGRADATION ; HETEROGENEOUS CATALYST ; COMPOSITE ELECTRODES
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science
WOS SubjectChemistry, Multidisciplinary ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS IDWOS:000529216500007
PublisherWILEY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/40366
Collection中国科学院过程工程研究所
Corresponding AuthorCherevan, Alexey S.; Streb, Carsten; Eder, Dominik
Affiliation1.Vienna Univ Technol, Inst Mat Chem, Getreidemarkt 9-BC-02, A-1060 Vienna, Austria
2.Ulm Univ, Inst Inorgan Chem 1, Albert Einstein Allee 11, D-89081 Ulm, Germany
3.Chinese Acad Sci, CAS Key Lab Green Proc & Engn, Inst Proc Engn, Beijing 100190, Peoples R China
4.Helmholtz Inst Ulm, Helmholtzstr 11, D-89081 Ulm, Germany
Recommended Citation
GB/T 7714
Cherevan, Alexey S.,Nandan, Sreejith P.,Roger, Isolda,et al. Polyoxometalates on Functional Substrates: Concepts, Synergies, and Future Perspectives[J]. ADVANCED SCIENCE,2020,7(8):23.
APA Cherevan, Alexey S.,Nandan, Sreejith P.,Roger, Isolda,Liu, Rongji,Streb, Carsten,&Eder, Dominik.(2020).Polyoxometalates on Functional Substrates: Concepts, Synergies, and Future Perspectives.ADVANCED SCIENCE,7(8),23.
MLA Cherevan, Alexey S.,et al."Polyoxometalates on Functional Substrates: Concepts, Synergies, and Future Perspectives".ADVANCED SCIENCE 7.8(2020):23.
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