CAS OpenIR
When hollow multishelled structures (HoMSs) meet metal-organic frameworks (MOFs)
Wang, Zumin1; Yang, Nailiang1,2; Wang, Dan1,2
2020-06-07
Source PublicationCHEMICAL SCIENCE
ISSN2041-6520
Volume11Issue:21Pages:5359-5368
AbstractHollow multishelled structures (HoMSs) have distinguished advantages, such as a large effective surface area, an optimized mass transport route, and a high loading capacity, but the fabrication of HoMSs has been a big challenge. In 2009, we developed a universal and facile method for HoMS fabrication, i.e., the sequential templating approach (STA). Progress in the synthetic methodology has enabled the study of HoMSs to develop and has made it a research hotspot in materials science. To date, HoMSs have shown their advantages in a wide range of applications, including catalysis, energy conversion and storage, drug delivery, etc. Based on the understanding in this field, we recently revealed the unique temporal-spatial ordering properties of HoMSs. Furthermore, we have been wondering if the structure of a HoMS can be modulated at the molecular level. Encouragingly, metal-organic frameworks (MOFs) are star materials with clearly defined molecular structures. The compositions, geometries, functionalities and topologies of MOFs have been well tuned by rational design. Integrating the unique properties of MOFs and HoMS could realize the systemic design of materials from the molecular to the micro-level, which would provide a series of advantages for various applications, such as developing high performance catalysts for cascade and/or selective catalysis, combining the reaction and separation process for multiple reactions, releasing drugs in a certain environment for smart medicine, and so on. We believe it is time to summarize the recent progress in the integration of MOFs and HoMSs, including HoMSs coated with MOFs, MOF-derived HoMSs, and MOFs with a hollow multishelled structure, and we also put forward our personal outlook in relation to the future opportunities and challenges in this emerging yet promising research field.
DOI10.1039/d0sc01284j
Language英语
WOS KeywordCRYSTAL ; MICROSPHERES ; COORDINATION ; PERFORMANCE ; SPHERES ; BATTERIES ; CATALYST ; DESIGN ; ANODES ; SNO2
Funding ProjectNational Natural Science Foundation of China[21590795] ; National Natural Science Foundation of China[21820102002] ; National Natural Science Foundation of China[21971244] ; Scientific Instrument Developing Project of the Chinese Academy of Sciences[YZ201623]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationNational Natural Science Foundation of China ; Scientific Instrument Developing Project of the Chinese Academy of Sciences
WOS IDWOS:000538158300001
PublisherROYAL SOC CHEMISTRY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/40923
Collection中国科学院过程工程研究所
Corresponding AuthorWang, Dan
Affiliation1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Wang, Zumin,Yang, Nailiang,Wang, Dan. When hollow multishelled structures (HoMSs) meet metal-organic frameworks (MOFs)[J]. CHEMICAL SCIENCE,2020,11(21):5359-5368.
APA Wang, Zumin,Yang, Nailiang,&Wang, Dan.(2020).When hollow multishelled structures (HoMSs) meet metal-organic frameworks (MOFs).CHEMICAL SCIENCE,11(21),5359-5368.
MLA Wang, Zumin,et al."When hollow multishelled structures (HoMSs) meet metal-organic frameworks (MOFs)".CHEMICAL SCIENCE 11.21(2020):5359-5368.
Files in This Item:
There are no files associated with this item.
Related Services
Recommend this item
Bookmark
Usage statistics
Export to Endnote
Google Scholar
Similar articles in Google Scholar
[Wang, Zumin]'s Articles
[Yang, Nailiang]'s Articles
[Wang, Dan]'s Articles
Baidu academic
Similar articles in Baidu academic
[Wang, Zumin]'s Articles
[Yang, Nailiang]'s Articles
[Wang, Dan]'s Articles
Bing Scholar
Similar articles in Bing Scholar
[Wang, Zumin]'s Articles
[Yang, Nailiang]'s Articles
[Wang, Dan]'s Articles
Terms of Use
No data!
Social Bookmark/Share
All comments (0)
No comment.
 

Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.