CAS OpenIR
Ionic-Liquid-Based Bioisoprene Recovery Process Design
Chen, Yuqiu1; Liu, Xinyan1,2; Kontogeorgis, Georgios M.1; Woodley, John M.1
2020-04-22
Source PublicationINDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
ISSN0888-5885
Volume59Issue:16Pages:7355-7366
AbstractBioisoprene, which can be produced from renewable feedstocks through fermentation, is a promising alternative to petroleum-derived isoprene. However, challenges including the selection of feasible recovery techniques for bioisoprene should be addressed to achieve economic and technical competitiveness. In this work, ionic liquids (ILs) are first introduced as solvents for the recovery of bioisoprene. To describe the thermodynamic behavior, the UNIFAC-IL model is first extended to the bioisoprene systems as it combines gas-organic chemicals in IL-containing systems. Using a computer-aided IL design (CAILD) method, six out of 248 742 structurally constrained ILs are screened as optimal candidates for their further performance evaluation. Simulation results indicate that all six ILs have much better process performance than that of the alternative, isopropyl myrisate. Moreover, [N-1,N-1,N-3,N-0][DMP] is identified as the best IL with the lowest solvent flow rate and the highest recovery ratio of isoprene. This work shows the potential of using ILs for the recovery of bioisoprene from fermentation off-gas.
DOI10.1021/acs.iecr.0c00146
Language英语
WOS KeywordUNIFAC GROUP-CONTRIBUTION ; PRESSURE PHASE-BEHAVIOR ; COMPUTER-AIDED-DESIGN ; CARBON-DIOXIDE ; RENEWABLE ISOPRENE ; COSMO-RS ; SOLUBILITY ; CO2 ; MODEL ; PREDICTION
Funding ProjectChina Scholarship Council[201708440264] ; Technical University of Denmark
WOS Research AreaEngineering
WOS SubjectEngineering, Chemical
Funding OrganizationChina Scholarship Council ; Technical University of Denmark
WOS IDWOS:000529151200009
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:3[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/40967
Collection中国科学院过程工程研究所
Corresponding AuthorWoodley, John M.
Affiliation1.Tech Univ Denmark, Dept Chem & Biochem Engn, DK-2800 Lyngby, Denmark
2.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, CAS Key Lab Green Proc & Engn, State Key Lab Multiphase Complex Syst,Inst Proc E, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Chen, Yuqiu,Liu, Xinyan,Kontogeorgis, Georgios M.,et al. Ionic-Liquid-Based Bioisoprene Recovery Process Design[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2020,59(16):7355-7366.
APA Chen, Yuqiu,Liu, Xinyan,Kontogeorgis, Georgios M.,&Woodley, John M..(2020).Ionic-Liquid-Based Bioisoprene Recovery Process Design.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,59(16),7355-7366.
MLA Chen, Yuqiu,et al."Ionic-Liquid-Based Bioisoprene Recovery Process Design".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 59.16(2020):7355-7366.
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