Knowledge Management System Of Institute of process engineering,CAS
| Effects of different temperature chars on distribution of pyrolysates for Naomaohu coal | |
| Liu, Zhutao1; Zhan, Jin-Hui1; Lai, Dengguo1; Zuo, Minghui2; Liu, Xiaoxing1 | |
| 2020-06-24 | |
| Source Publication | JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY
 |
| ISSN | 1388-6150 |
| Pages | 10 |
| Abstract | Intrinsic characteristics of Naomaohu coal pyrolysis in a two-stage fixed-bed reactor have been investigated in this study. The pyrolysates were detected by the simulated distillation, ultimate analysis and GC-MS to analyze the effect of different temperature chars on pyrolysis volatiles. The results showed that the slight secondary reactions occurred when the volatiles flowed through the 100-400 degrees C char layer, the yield of pyrolysis gas increased slightly, the tar yield had a little decrease, the atomic H/C ratio was higher than that of blank contrast experiment, and the quality of oil increased. Under the action of 500-900 degrees C char layer, the drastic secondary reactions of the volatiles occurred, the yield of pyrolysis gas increased obviously, and the yield and quality of oil decreased. The results of two-stage experiments with and without char effect were similar to the temperature change, indicating that temperature played a major role in affecting the distribution of pyrolysates. Whereas char was beneficial for the content and quality of light oil in the low-temperature range, the process of volatiles through the semi-coke layer enhanced H(2)and CH(4)yield during the total temperature range. Char also had an adsorption action, which gradually weakened with the temperature increased. |
| Keyword | Coal Pyrolysis Char Secondary reaction Temperature |
| DOI | 10.1007/s10973-020-09934-y |
| Language | 英语 |
| WOS Keyword | HIGH-QUALITY TAR ; SECONDARY REACTIONS ; FLASH PYROLYSIS ; BEHAVIOR ; DEVOLATILIZATION ; PRESSURE ; PRODUCTS ; KINETICS ; GAS ; OIL |
| Funding Project | National Natural Science Foundation of China[21875255] ; Heilongjiang Education Department Project[1354ZD001] ; MuDanjiang Normal University National Project Cultivation Project[GP2018002] |
| WOS Research Area | Thermodynamics ; Chemistry |
| WOS Subject | Thermodynamics ; Chemistry, Analytical ; Chemistry, Physical |
| Funding Organization | National Natural Science Foundation of China ; Heilongjiang Education Department Project ; MuDanjiang Normal University National Project Cultivation Project |
| WOS ID | WOS:000543024800002 |
| Publisher | SPRINGER |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.ipe.ac.cn/handle/122111/41220 |
| Collection | 中国科学院过程工程研究所 |
| Corresponding Author | Zhan, Jin-Hui; Liu, Xiaoxing |
| Affiliation | 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 2.Mudanjiang Normal Univ, Coll Chem & Chem Engn, Mudanjing 157012, Peoples R China |
| Recommended Citation GB/T 7714 | Liu, Zhutao,Zhan, Jin-Hui,Lai, Dengguo,et al. Effects of different temperature chars on distribution of pyrolysates for Naomaohu coal[J]. JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY,2020:10. |
| APA | Liu, Zhutao,Zhan, Jin-Hui,Lai, Dengguo,Zuo, Minghui,&Liu, Xiaoxing.(2020).Effects of different temperature chars on distribution of pyrolysates for Naomaohu coal.JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY,10. |
| MLA | Liu, Zhutao,et al."Effects of different temperature chars on distribution of pyrolysates for Naomaohu coal".JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY (2020):10. |
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