CAS OpenIR
Highly enhanced electrocatalytic activity of nano-TiO2/Ti membrane electrode for phenol wastewater treatment
Xu, Jiaxin1; Liang, Xiaoping1; Fan, Xiaowei2; Song, Yuxi1; Zhao, Zenghua3; Hua, Junyuan1; Liu, Chuan1; Li, Jianxin1
2020-07-13
Source PublicationJOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
ISSN0957-4522
Pages10
AbstractNano-TiO2/Ti composite membrane electrodes with different morphological TiO2, including nanoparticles (NP), nanowires (NW), and nanosheets (NS), were successfully prepared by hydrothermal reaction process under different hydrothermal temperatures. The effects of the morphology of TiO(2)catalyst on the structure and properties of TiO2/Ti composite membrane electrodes were evaluated by X-ray diffraction, field-emission scanning electronic microscopy, and X-ray Photoelectron spectroscopy. Compared with both NP-TiO2/Ti and NS-TiO2/Ti, it was found that NW-TiO2/Ti had lower charge transfer resistance and larger peak current. Electrocatalytic membrane reactor (ECMR) has been successfully designed for the treatment of phenolic wastewater, which is assembled with a TiO2/Ti composite membrane electrode as an anode. ECMR with NW-TiO2/Ti had the best electrochemical activity, whose phenol removal rate was 93.13%, but was 84.25%, 82.72%, and 46.86% in the case of NS-TiO2/Ti, NP-TiO2/Ti, and Ti electrodes, respectively. Meanwhile, comparing with others, ECMR with NW-TiO2/Ti had the lowest energy consumption (0.756 kWh/kgCOD). The results demonstrated that the excellent electrochemical performance of ECMR with NW-TiO2/Ti was deeply related to the nanowire morphology of TiO(2)catalyst coated on Ti substrate electrode, which was mainly reflected in the larger effective electrocatalytic surface area and higher electron transfer rate of NW-TiO2/Ti composite membrane electrode.
DOI10.1007/s10854-020-03907-5
Language英语
WOS KeywordELECTROCHEMICAL OXIDATION ; EFFICIENT ELECTROCATALYST ; PHOTOCATALYTIC ACTIVITY ; COMPOSITE ; OXIDE ; NANOPARTICLES ; DEGRADATION ; PERFORMANCE ; MORPHOLOGY ; REACTOR
Funding ProjectNational Natural Science Foundation of China[21576208] ; Science and Technology Planning Projects of Tianjin[17JCYBJC19800] ; Program for Innovative Research Team in University of Ministry of Education of China[IRT-17R80] ; Tianjin Science and Technology Planning Project[18PTZWHZ00210]
WOS Research AreaEngineering ; Materials Science ; Physics
WOS SubjectEngineering, Electrical & Electronic ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
Funding OrganizationNational Natural Science Foundation of China ; Science and Technology Planning Projects of Tianjin ; Program for Innovative Research Team in University of Ministry of Education of China ; Tianjin Science and Technology Planning Project
WOS IDWOS:000548260800004
PublisherSPRINGER
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/41421
Collection中国科学院过程工程研究所
Corresponding AuthorLiang, Xiaoping; Li, Jianxin
Affiliation1.Tianjin Polytech Univ, Sch Mat Sci & Engn, Natl Ctr Int Joint Res Membrane Sci & Technol, State Key Lab Separat Membranes & Membrane Proc, Tianjin 300387, Peoples R China
2.Tianjin SYP Engn Glass Co Ltd, Tianjin 300409, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiph Ase Complex Syst, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Xu, Jiaxin,Liang, Xiaoping,Fan, Xiaowei,et al. Highly enhanced electrocatalytic activity of nano-TiO2/Ti membrane electrode for phenol wastewater treatment[J]. JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,2020:10.
APA Xu, Jiaxin.,Liang, Xiaoping.,Fan, Xiaowei.,Song, Yuxi.,Zhao, Zenghua.,...&Li, Jianxin.(2020).Highly enhanced electrocatalytic activity of nano-TiO2/Ti membrane electrode for phenol wastewater treatment.JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,10.
MLA Xu, Jiaxin,et al."Highly enhanced electrocatalytic activity of nano-TiO2/Ti membrane electrode for phenol wastewater treatment".JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS (2020):10.
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