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Conversion of palmitic acid to jet fuel components over Mo/H-ZSM-22 bi-functional catalysts with high carbon reservation
Zhang, Jimei1,3; Shi, Yanchun1; Cao, Hongbin1; Wu, Yulong2; Yang, Mingde2
2020-11-25
Source PublicationAPPLIED CATALYSIS A-GENERAL
ISSN0926-860X
Volume608Pages:10
AbstractThe optimal preparation conditions of Mo/H-ZSM-22 bi-functional catalysts were obtained via the sublimation phenomenon of MoO3 at high calcination temperatures, which was beneficial for the well-dispersion of MoOx species with 5-10 nm particles. High reduction temperature enhanced the reduction from Mo6+ to Mo4+ and even from Mo4+ to Mo, which would be beneficial for iso-alkanes formation with higher carbon reservation. Importantly, 89.3 % selectivity of C-16 alkanes of which 61.7 % were iso-C-16 alkanes were obtained with complete deoxygenation of palmitic acid, which was the highest selectivity of C-16 alkanes over Mo/H-ZSM-22 bi-functional catalyst prepared at a calcination temperature of 550 degrees C and at a reduction temperature of 600 degrees C. The results would offer a novel candidate of bi-functional catalysts for upgrading of microalgae-based bio-oil to high value jet fuel components with high selectivity of iso-alkanes and carbon reservation.
KeywordMo/H-ZSM-22 Palmitic acid Hydrodeoxygenation Isomerization
DOI10.1016/j.apcata.2020.117847
Language英语
WOS KeywordACTIVATED CARBON ; MICROALGAE OIL ; RAPESEED OIL ; STEARIC-ACID ; FATTY-ACIDS ; NI ; HYDRODEOXYGENATION ; DEOXYGENATION ; DIESEL ; MO
Funding ProjectNational Science Foundation of China[21838006] ; National Science Foundation of China[21776159] ; National Science Foundation of China[21576155]
WOS Research AreaChemistry ; Environmental Sciences & Ecology
WOS SubjectChemistry, Physical ; Environmental Sciences
Funding OrganizationNational Science Foundation of China
WOS IDWOS:000592362200002
PublisherELSEVIER
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/42690
Collection中国科学院过程工程研究所
Corresponding AuthorShi, Yanchun; Wu, Yulong
Affiliation1.Chinese Acad Sci, Inst Proc Engn, CAS Key Lab Green Proc & Engn, Beijing 100190, Peoples R China
2.Tsinghua Univ, Inst Nucl & New Energy Technol, Beijing 100084, Peoples R China
3.Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Jimei,Shi, Yanchun,Cao, Hongbin,et al. Conversion of palmitic acid to jet fuel components over Mo/H-ZSM-22 bi-functional catalysts with high carbon reservation[J]. APPLIED CATALYSIS A-GENERAL,2020,608:10.
APA Zhang, Jimei,Shi, Yanchun,Cao, Hongbin,Wu, Yulong,&Yang, Mingde.(2020).Conversion of palmitic acid to jet fuel components over Mo/H-ZSM-22 bi-functional catalysts with high carbon reservation.APPLIED CATALYSIS A-GENERAL,608,10.
MLA Zhang, Jimei,et al."Conversion of palmitic acid to jet fuel components over Mo/H-ZSM-22 bi-functional catalysts with high carbon reservation".APPLIED CATALYSIS A-GENERAL 608(2020):10.
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