CFD Simulation of a Fluid-Solid Non-Catalytic Reaction Based on a Structure-Based Mass Transfer Model: Shrinking Spherical Reaction

doi:10.1021/acs.iecr.0c04409

CAS OpenIR

	CFD Simulation of a Fluid-Solid Non-Catalytic Reaction Based on a Structure-Based Mass Transfer Model: Shrinking Spherical Reaction
	Zou, Zheng 1,2; Zhu, Jingyi 1,2; Jia, Jibin 1,2; Du, Zhan 1; Wang, Qiao 3; Zhu, Qingshan 1,2; Li, Hongzhong 1,2
	2020-11-11
Source Publication	INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
ISSN	0888-5885
Volume	59 Issue:45 Pages:19989-19998
Abstract	To forecast the mass transfer behavior in consideration of noncatalytic solid reaction characteristics with the shrinking spherical model (SPM), a structure-based mass transfer model taking account of the gas-solid mass exchange within both the emulsion and bubble/interphase phases is built and coupled with computational fluid dynamics (CFD) to predict the carbochlorination of TiO2 with a binary gas-solid phase system. Based on the validation through comparing with the experimental data, the simulation gives a comprehensive understanding and deep analysis of the gas-solid reaction that is helpful for the design and optimization of a non-catalytic fluidized reactor. It is concluded that the fluidized mass transfer process with a heterogeneous flow structure is not only affected by the chemical reaction rate but also dependent on local flow parameters.
DOI	10.1021/acs.iecr.0c04409
Language	英语
Funding Project	National Natural Science Foundation of China[21878304] ; National Natural Science Foundation of China[21736010] ; National Natural Science Foundation of China[21908227] ; Science Fund for Creative Research Groups of the National Natural Science Foundation of China[21921005] ; State Key Laboratory of Multiphase Complex Systems[MPCS-2019-A-07]
WOS Research Area	Engineering
WOS Subject	Engineering, Chemical
Funding Organization	National Natural Science Foundation of China ; Science Fund for Creative Research Groups of the National Natural Science Foundation of China ; State Key Laboratory of Multiphase Complex Systems
WOS ID	WOS:000592479200016
Publisher	AMER CHEMICAL SOC
Citation statistics
Document Type	期刊论文
Identifier	http://ir.ipe.ac.cn/handle/122111/43168
Collection	中国科学院过程工程研究所
Corresponding Author	Zou, Zheng; Zhu, Qingshan
Affiliation	1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multi Phase Complex Syst, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Comp Network Informat Ctr, Beijing 100190, Peoples R China
Recommended Citation GB/T 7714	Zou, Zheng,Zhu, Jingyi,Jia, Jibin,et al. CFD Simulation of a Fluid-Solid Non-Catalytic Reaction Based on a Structure-Based Mass Transfer Model: Shrinking Spherical Reaction[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2020,59(45):19989-19998.
APA	Zou, Zheng.,Zhu, Jingyi.,Jia, Jibin.,Du, Zhan.,Wang, Qiao.,...&Li, Hongzhong.(2020).CFD Simulation of a Fluid-Solid Non-Catalytic Reaction Based on a Structure-Based Mass Transfer Model: Shrinking Spherical Reaction.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,59(45),19989-19998.
MLA	Zou, Zheng,et al."CFD Simulation of a Fluid-Solid Non-Catalytic Reaction Based on a Structure-Based Mass Transfer Model: Shrinking Spherical Reaction".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 59.45(2020):19989-19998.

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