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Electrochemical and Photoelectrochemical Water Oxidation for Hydrogen Peroxide Production
Xue, Yudong1,5; Wang, Yunting2; Pan, Zhenhua3; Sayama, Kazuhiro4
2021-01-21
Source PublicationANGEWANDTE CHEMIE-INTERNATIONAL EDITION
ISSN1433-7851
Pages13
AbstractHydrogen peroxide (H2O2), as a green fuel and oxidant, has drawn increasing attention in the energy and environmental research. Compared with the traditional anthraquinone process, the electrochemical (EC) and photoelectrochemical (PEC) syntheses of H2O2 are cost-effective and environmentally friendly. In order to construct membraneless EC/PEC devices for the full H2O2 synthesis, anodic H2O2 production by water oxidation, which is less developed than cathodic H2O2 generation, is highly desirable. Here, we review recent developments for the EC/PEC H2O2 production by water oxidation, including fundamental aspects, benchmarking activity evaluation, material/catalyst selection, and strategies for increasing selectivity, efficiency, and accumulation. Furthermore, we discuss the challenges and outlook of water oxidation for H2O2 production, especially device-level development, accumulation and stability, and industrial applications. Our review is intended to stimulate studies further improving EC/PEC H2O2 production.
Keywordelectrochemistry hydrogen peroxide photoelectrochemistry water oxidation
DOI10.1002/anie.202011215
Language英语
Funding ProjectChina Scholarship Council (CSC)[201906430035] ; International Joint Research Program for Innovative Energy Technology ; JSPS KAKENHI[JP17H06436]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationChina Scholarship Council (CSC) ; International Joint Research Program for Innovative Energy Technology ; JSPS KAKENHI
WOS IDWOS:000610994100001
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/43321
Collection中国科学院过程工程研究所
Corresponding AuthorXue, Yudong; Pan, Zhenhua; Sayama, Kazuhiro
Affiliation1.Korea Univ, Coll Engn, Seoul 136701, South Korea
2.China Univ Min & Technol Beijing, Sch Chem & Environm Engn, Beijing 100083, Peoples R China
3.Chuo Univ, Dept Appl Chem, Fac Sci & Technol, Bunkyo Ku, 1-13-27 Kasuga, Tokyo 1128551, Japan
4.Natl Inst Adv Ind Sci & Technol, Global Zero Emiss Res Ctr GZR, Cent 5,1-1-1 Higashi, Tsukuba, Ibaraki 3058565, Japan
5.Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Xue, Yudong,Wang, Yunting,Pan, Zhenhua,et al. Electrochemical and Photoelectrochemical Water Oxidation for Hydrogen Peroxide Production[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2021:13.
APA Xue, Yudong,Wang, Yunting,Pan, Zhenhua,&Sayama, Kazuhiro.(2021).Electrochemical and Photoelectrochemical Water Oxidation for Hydrogen Peroxide Production.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,13.
MLA Xue, Yudong,et al."Electrochemical and Photoelectrochemical Water Oxidation for Hydrogen Peroxide Production".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021):13.
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