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Study on Combustion Performance of Mn-Based Binary Carrier Catalyst for Ventilation Air Methane
Xu Xin1; Liu Wenge1; Qi Jian2,3; Yu Lei1; Han Jiaye1; Li Zhi1
2020-12-30
Source PublicationCHINA PETROLEUM PROCESSING & PETROCHEMICAL TECHNOLOGY
ISSN1008-6234
Volume22Issue:4Pages:26-34
AbstractLa-Al2O3 and Ce-Al2O3 binary monolithic column materials with dual functions of carrier and promoter were prepared in one-step by the sol-gel method. Using the as-synthesized binary monolithic column materials as carrier, the 9%Mn/ M-Al2O3 (M=La/Ce) catalyst was prepared by the impregnation method. The binary carrier and catalyst were characterized by BET, SEM, XRD, H-2-TPR, and O-2-TPD techniques, and the methane combustion performance was tested in a micro fixed-bed reactor. Results showed that the Mn-based binary carrier catalyst with dual functions of carrier and promoter had higher catalytic activity than that with single alumina acting as the carrier. The catalyst activity gradually increased with an increasing content of La, while there was no significant effect with the increase in Ce content. When the ratio of La content in La-Al2O3 is 11%, 1% of methane contained in the ventilation air can be completely converted over the 9%Mn/11% La-Al2O3 catalyst at a temperature as low as 550 degrees C.
Keywordbinary carrier catalytic combustion VAM Mn/La-Al2O3 Mn/Ce-Al2O3
Language英语
WOS KeywordSOL-GEL PROCESS ; OXIDATION
Funding ProjectNational Youth Science Foundation[51704086] ; National Natural Science Foundation of China[51772294] ; National Natural Science Foundation of China[51972306]
WOS Research AreaEnergy & Fuels ; Engineering
WOS SubjectEnergy & Fuels ; Engineering, Chemical ; Engineering, Petroleum
Funding OrganizationNational Youth Science Foundation ; National Natural Science Foundation of China
WOS IDWOS:000616418400004
PublisherCHINA PETROLEUM PROCESSING & PETROCHEMICAL TECHNOLOGY PRESS
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/43375
Collection中国科学院过程工程研究所
Corresponding AuthorXu Xin; Liu Wenge
Affiliation1.China Coal Informat Inst, Beijing 100029, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Xu Xin,Liu Wenge,Qi Jian,et al. Study on Combustion Performance of Mn-Based Binary Carrier Catalyst for Ventilation Air Methane[J]. CHINA PETROLEUM PROCESSING & PETROCHEMICAL TECHNOLOGY,2020,22(4):26-34.
APA Xu Xin,Liu Wenge,Qi Jian,Yu Lei,Han Jiaye,&Li Zhi.(2020).Study on Combustion Performance of Mn-Based Binary Carrier Catalyst for Ventilation Air Methane.CHINA PETROLEUM PROCESSING & PETROCHEMICAL TECHNOLOGY,22(4),26-34.
MLA Xu Xin,et al."Study on Combustion Performance of Mn-Based Binary Carrier Catalyst for Ventilation Air Methane".CHINA PETROLEUM PROCESSING & PETROCHEMICAL TECHNOLOGY 22.4(2020):26-34.
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