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A general strategy to prepare atomically dispersed biomimetic catalysts based on host-guest chemistry
Han, Xiao1; Chen, Zheng2,3; Chen, Wenxing2,4; Lv, Chunlin5,6; Ji, Yongjun7,8; Li, Jing8; Cheong, Weng-Chon2; Lei, Xiaojuan1; Peng, Qing2; Chen, Chen2; Wang, Dingsheng2; Lian, Chao4,9; Li, Yadong2
2021-02-21
Source PublicationCHEMICAL COMMUNICATIONS
ISSN1359-7345
Volume57Issue:15Pages:1895-1898
Abstract

Herein, we report a general strategy based on host-guest interactions to fabricate atomically dispersed biomimetic catalysts, which were evaluated by diboration of phenylacetylene. The structure and function of these mimics are quite similar to those of enzymes, namely, the atomically dispersed metal serves as an active site, the external macromolecular structure plays a role as an enzyme catalytic pocket to stabilize the reaction intermediates and the interactions between the intermediates and functional groups near to the active site can reduce the reaction activation energy.

DOI10.1039/d0cc07119f
Language英语
Funding ProjectNational Natural Science Foundation of China[21701007] ; National Natural Science Foundation of China[21801015]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationNational Natural Science Foundation of China
WOS IDWOS:000620719300009
PublisherROYAL SOC CHEMISTRY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/47888
Collection中国科学院过程工程研究所
Corresponding AuthorLian, Chao
Affiliation1.Beijing Jiaotong Univ, Sch Sci, Dept Chem, Beijing 100044, Peoples R China
2.Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China
3.Anhui Normal Univ, Coll Chem & Mat Sci, Key Lab Funct Mol Solids, Anhui Key Lab Mol Based Mat,Minist Educ, Wuhu 241000, Peoples R China
4.Being Inst Technol, Beijing Key Lab Construct Tailorable Adv Funct Ma, Sch Mat Sci & Engn, Beijing 100081, Peoples R China
5.Minzu Univ China, Sch Pharm, Beijing 100081, Peoples R China
6.Minzu Univ China, Ctr Translat Neurosci, Beijing 100081, Peoples R China
7.Beijing Technol & Business Univ, Sch Light Ind, Beijing 100048, Peoples R China
8.Chinese Acad Sci, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing 100190, Peoples R China
9.Beijing Single Atom Site Catalysis Technol Co Ltd, Beijing 100094, Peoples R China
Recommended Citation
GB/T 7714
Han, Xiao,Chen, Zheng,Chen, Wenxing,et al. A general strategy to prepare atomically dispersed biomimetic catalysts based on host-guest chemistry[J]. CHEMICAL COMMUNICATIONS,2021,57(15):1895-1898.
APA Han, Xiao.,Chen, Zheng.,Chen, Wenxing.,Lv, Chunlin.,Ji, Yongjun.,...&Li, Yadong.(2021).A general strategy to prepare atomically dispersed biomimetic catalysts based on host-guest chemistry.CHEMICAL COMMUNICATIONS,57(15),1895-1898.
MLA Han, Xiao,et al."A general strategy to prepare atomically dispersed biomimetic catalysts based on host-guest chemistry".CHEMICAL COMMUNICATIONS 57.15(2021):1895-1898.
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