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Achieving high singlet-oxygen generation by applying the heavy-atom effect to thermally activated delayed fluorescent materials | |
Xiao, Ya-Fang1,2,3,4; Chen, Jia-Xiong1,2,3,4; Chen, Wen-Cheng5; Zheng, Xiuli3,4,6; Cao, Chen1,2,3,4; Tan, Jihua1,2,3,4; Cui, Xiao1,2,3,4; Yuan, Zhanxiang5; Ji, Shaomin5; Lu, Guihong7; Liu, Weimin3,4,6; Wang, Pengfei3,4,6; Li, Shengliang1,2,3,4; Lee, Chun-Sing1,2,3,4 | |
2021-04-12 | |
Source Publication | CHEMICAL COMMUNICATIONS
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ISSN | 1359-7345 |
Pages | 4 |
Abstract | A bromine-substituted thermally activated delayed fluorescent (TADF) molecule AQCzBr(2) is designed with both small singlet-triplet splitting (Delta E-ST) and increased spin-orbit coupling (SOC) to boost intersystem crossing (ISC) for singlet oxygen generation. AQCzBr(2) nanoparticles (NPs) demonstrate high productivity of singlet oxygen generation (phi(Delta) = 0.91) which allows highly efficient photodynamic therapy toward cancer cells. |
DOI | 10.1039/d0cc08323b |
Language | 英语 |
Funding Project | City University of Hong Kong[JLFS/P-101/18] ; ITF[ITS/219/19] ; University Grants Committee/Research Grants Council of the Hong Kong Special Administrative Region, China[JLFS/P-101/18] ; Research Grants Council of the Hong Kong Special Administrative Region, China[11300418] ; ARG-CityU Applied Research Grant[9667160] ; National Natural Science Foundation of China[52003058] |
WOS Research Area | Chemistry |
WOS Subject | Chemistry, Multidisciplinary |
Funding Organization | City University of Hong Kong ; ITF ; University Grants Committee/Research Grants Council of the Hong Kong Special Administrative Region, China ; Research Grants Council of the Hong Kong Special Administrative Region, China ; ARG-CityU Applied Research Grant ; National Natural Science Foundation of China |
WOS ID | WOS:000641059700001 |
Publisher | ROYAL SOC CHEMISTRY |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.ipe.ac.cn/handle/122111/48428 |
Collection | 中国科学院过程工程研究所 |
Corresponding Author | Chen, Wen-Cheng; Lu, Guihong; Li, Shengliang; Lee, Chun-Sing |
Affiliation | 1.City Univ Hong Kong, Ctr Super Diamond & Adv Films COSDAF, Hong Kong 999077, Peoples R China 2.City Univ Hong Kong, Dept Chem, Hong Kong 999077, Peoples R China 3.City Univ Hong Kong, Joint Lab Nanoorgan Funct Mat & Devices TIPC, Kowloon, Hong Kong, Peoples R China 4.City Univ Hong Kong, CityU, Kowloon, Hong Kong, Peoples R China 5.Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Peoples R China 6.Chinese Acad Sci, Tech Inst Phys & Chem, Beijing 100190, Peoples R China 7.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China |
Recommended Citation GB/T 7714 | Xiao, Ya-Fang,Chen, Jia-Xiong,Chen, Wen-Cheng,et al. Achieving high singlet-oxygen generation by applying the heavy-atom effect to thermally activated delayed fluorescent materials[J]. CHEMICAL COMMUNICATIONS,2021:4. |
APA | Xiao, Ya-Fang.,Chen, Jia-Xiong.,Chen, Wen-Cheng.,Zheng, Xiuli.,Cao, Chen.,...&Lee, Chun-Sing.(2021).Achieving high singlet-oxygen generation by applying the heavy-atom effect to thermally activated delayed fluorescent materials.CHEMICAL COMMUNICATIONS,4. |
MLA | Xiao, Ya-Fang,et al."Achieving high singlet-oxygen generation by applying the heavy-atom effect to thermally activated delayed fluorescent materials".CHEMICAL COMMUNICATIONS (2021):4. |
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Achieving high singl(3057KB) | 期刊论文 | 出版稿 | 限制开放 | CC BY-NC-SA | Application Full Text |
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