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Ultrafine Ir nanoparticles decorated on FeP/FeOOH with abundant interfaces via a facile corrosive approach for alkaline water-splitting
Zhao, Zongshi1; Jin, Wei3; Xu, Li5; Wang, Chan1; Zhang, Yang4; Wu, Zexing2
2021-05-28
Source PublicationJOURNAL OF MATERIALS CHEMISTRY A
ISSN2050-7488
Volume9Issue:20Pages:12074-12079
AbstractIn order to generate clean hydrogen fuel, it is necessary to exploit bifunctional catalysts with high activity and excellent stability for overall water-splitting. Herein, we develop ultrafine Ir nanoparticles coupled with FeP/FeOOH with abundant interfaces on iron foam (FF) via facile corrosive strategies. The ingeniously designed catalyst structure not only exposes abundant active centers, but also enhances the electron transport efficiently. Thus, the FF-NaCl-Ir-P catalyst exhibits outstanding catalytic activities for the OER (169 mV at 10 mA cm(-2)) and HER (69 mV at 10 mA cm(-2)) in 1 M KOH, which was better than most of the previously reported catalysts. For water-splitting, it only needs 1.47 V to reach 10 mA cm(-2), and its performance hardly deteriorates after 50 hours test at a large-current density of 1000 mA cm(-2). The overall water-splitting can also be motivated by simple sustainable energy, such as solar, wind and thermal energies.
DOI10.1039/d1ta02658e
Language英语
WOS KeywordLAYERED DOUBLE HYDROXIDE ; PRUSSIAN BLUE ANALOG ; BIFUNCTIONAL ELECTROCATALYST ; HIGHLY EFFICIENT ; OXYGEN ; CATALYSTS ; NANOSHEETS ; PHOSPHIDE ; FE
Funding ProjectNatural Science Foundation of China[22002068] ; Natural Science Foundation of China[51973083] ; National Key R&D Program of China[2018YFC1900505] ; Natural Science Foundation of Shandong Province of China[ZR2019BB002] ; National.rst-class discipline program of Food Science and Technology[JUFSTR20180301] ; Fundamental Research Funds for the Central Universities[JUSRP22027] ; Doctoral Fund of QUST[010022873] ; Tongji Hundred Talents Program
WOS Research AreaChemistry ; Energy & Fuels ; Materials Science
WOS SubjectChemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary
Funding OrganizationNatural Science Foundation of China ; National Key R&D Program of China ; Natural Science Foundation of Shandong Province of China ; National.rst-class discipline program of Food Science and Technology ; Fundamental Research Funds for the Central Universities ; Doctoral Fund of QUST ; Tongji Hundred Talents Program
WOS IDWOS:000651127800001
PublisherROYAL SOC CHEMISTRY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/48564
Collection中国科学院过程工程研究所
Corresponding AuthorWang, Chan; Zhang, Yang; Wu, Zexing
Affiliation1.Jiangnan Univ, Sch Chem & Mat Engn, Wuxi 214122, Jiangsu, Peoples R China
2.Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, State Key Lab Base Ecochem Engn, 53 Zhengzhou Rd, Qingdao 266042, Peoples R China
3.Tongji Univ, State Key Lab Pollut Control & Resources Reuse, Sch Environm Sci & Engn, 1239 Siping Rd, Shanghai 200092, Peoples R China
4.Chinese Acad Sci, Inst Proc Engn, 1st Ber Er Tiao Zhongguancun, Beijing 100190, Peoples R China
5.Shanghai Inst Planned Parenthood Res, 2140 Xietu Rd, Shanghai 200032, Peoples R China
Recommended Citation
GB/T 7714
Zhao, Zongshi,Jin, Wei,Xu, Li,et al. Ultrafine Ir nanoparticles decorated on FeP/FeOOH with abundant interfaces via a facile corrosive approach for alkaline water-splitting[J]. JOURNAL OF MATERIALS CHEMISTRY A,2021,9(20):12074-12079.
APA Zhao, Zongshi,Jin, Wei,Xu, Li,Wang, Chan,Zhang, Yang,&Wu, Zexing.(2021).Ultrafine Ir nanoparticles decorated on FeP/FeOOH with abundant interfaces via a facile corrosive approach for alkaline water-splitting.JOURNAL OF MATERIALS CHEMISTRY A,9(20),12074-12079.
MLA Zhao, Zongshi,et al."Ultrafine Ir nanoparticles decorated on FeP/FeOOH with abundant interfaces via a facile corrosive approach for alkaline water-splitting".JOURNAL OF MATERIALS CHEMISTRY A 9.20(2021):12074-12079.
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